• Photonics Research
  • Vol. 6, Issue 2, 99 (2018)
Daquan Yang1、2、†, Fei Gao3、†, Qi-Tao Cao3, Chuan Wang2, Yuefeng Ji1、2, and Yun-Feng Xiao3、4、*
Author Affiliations
  • 1School of Information and Communication Engineering, Beijing University of Posts and Telecommunications, Beijing 100876, China
  • 2State Key Laboratory of Information Photonics and Optical Communications, Beijing University of Posts and Telecommunications, Beijing 100876, China
  • 3State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University, Collaborative Innovation Center of Quantum Matter, Beijing 100871, China
  • 4Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan, Shanxi 030006, China
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    DOI: 10.1364/PRJ.6.000099 Cite this Article Set citation alerts
    Daquan Yang, Fei Gao, Qi-Tao Cao, Chuan Wang, Yuefeng Ji, Yun-Feng Xiao. Single nanoparticle trapping based on on-chip nanoslotted nanobeam cavities[J]. Photonics Research, 2018, 6(2): 99 Copy Citation Text show less

    Abstract

    Optical trapping techniques are of great interest since they have the advantage of enabling the direct handling of nanoparticles. Among various optical trapping systems, photonic crystal nanobeam cavities have attracted great attention for integrated on-chip trapping and manipulation. However, optical trapping with high efficiency and low input power is still a big challenge in nanobeam cavities because most of the light energy is confined within the solid dielectric region. To this end, by incorporating a nanoslotted structure into an ultracompact one-dimensional photonic crystal nanobeam cavity structure, we design a promising on-chip device with ultralarge trapping potential depth to enhance the optical trapping characteristic of the cavity. In this work, we first provide a systematic analysis of the optical trapping force for an airborne polystyrene (PS) nanoparticle trapped in a cavity model. Then, to validate the theoretical analysis, the numerical simulation proof is demonstrated in detail by using the three-dimensional finite element method. For trapping a PS nanoparticle of 10 nm radius within the air-slot, a maximum trapping force as high as 8.28 nN/mW and a depth of trapping potential as large as 1.15×105 kBT mW 1 are obtained, where kB is the Boltzmann constant and T is the system temperature. We estimate a lateral trapping stiffness of 167.17 pN·nm 1· mW 1 for a 10 nm radius PS nanoparticle along the cavity x-axis, more than two orders of magnitude higher than previously demonstrated on-chip, near field traps. Moreover, the threshold power for stable trapping as low as 0.087 μW is achieved. In addition, trapping of a single 25 nm radius PS nanoparticle causes a 0.6 nm redshift in peak wavelength. Thus, the proposed cavity device can be used to detect single nanoparticle trapping by monitoring the resonant peak wavelength shift. We believe that the architecture with features of an ultracompact footprint, high integrability with optical waveguides/circuits, and efficient trapping demonstrated here will provide a promising candidate for developing a lab-on-a-chip device with versatile functionalities.

    1. INTRODUCTION

    To date, the ability to micromanipulate nanoscopic particles precisely is critical for the development of active nanosystems [1]. Over the past several decades, optical trapping, the force applied on a nanoscopic particle with noncontact and nondestructive features, has exceeded mechanical force in many applications ranging from physics to biochemical; it also provides an all-optical method that allows one to manipulate nanoparticles ranging in size from several micrometers to a few nanometers [25]. Since the original experiments reported in Ashkin’s pioneering work [6] on laser-induced optical trapping and the manipulation of micrometer-sized dielectric microspheres, optical or laser tweezing techniques [7] have been used for a variety of application areas, such as optical chromatography, flow cytometry, and directed assembly.

    So far, via optical trapping, a large number of different nanoparticles including dielectric/metallic nanoparticles, single cells, and even single atoms can be manipulated [810]. Particularly, to further establish trapping nanoparticles with lower input powers, a number of new, near-field optical manipulation techniques, such as optical nanofibers [1113], photonic crystal (PC) fibers [14,15], whispering gallery mode carousels [1620], plasmonic tweezers [2124], solid waveguides [25,26], slot waveguides [27,28], microring resonators [29], photonic crystal waveguides [3032], and photonic crystal cavities [3350], have been developed to exploit the strong spatial field gradient forces and to increase the field amplitude inside the devices. Among these, photonic crystal cavities have been investigated as advantageous platforms for cavity-enhanced optical trapping and sensing due to their advantage in high Q/V, where Q is the quality factor and V is the cavity mode volume. Particularly, compared with two-dimensional (2D) PC cavities [3339], one-dimensional (1D) PC nanobeam cavities [4050] have attracted great attention for integrated on-chip trapping and manipulation due to their attractive properties of ultracompact footprints and convenient integration with bus-waveguides. Examples of such systems include a 1D PC cavity with waist design for efficient trapping and nanoparticle detection presented by Lin et al., where an optical trapping force of 2.3 pN/mW for a 100 nm diameter polystyrene (PS) nanoparticle was observed [40]; Serey et al. theoretically showed that nanoparticles as small as 7.7 nm in diameter can be trapped with a trapping potential depth of 500  kBT when the input power is 10 mW, where kB is the Boltzmann constant and T is the system temperature [41]; Mandal et al. presented a class of silicon 1D PC resonant optical trapping for nanomanipulation and observed that the maximum trapping force of 700 pN/W for a 100 nm diameter PS nanoparticle was achieved [42]; Han and Shi theoretically showed that an optical trapping force as high as 300 pN/mW for a 200 nm diameter PS nanoparticle in a 1D PC system was achieved [49].

    However, among the 1D-PC-cavity-based optical trapping schemes mentioned above, the fact is that the trapped objects only interact with a minor portion of total light energy within the cavity because most of the light energy is confined within the solid core of the high-index dielectric region. This limits these systems from precisely manipulating smaller nanoscopic matter due to the low efficiency interactions between the trapped objects and the optical field. Thus, usually to achieve a large optical trapping force to manipulate nanoparticles precisely, a high input optical power is needed. However, the high input power can affect or even damage the trapped objects (e.g., small biomolecules) due to the optical-absorption-induced temperature increasing, which practically limits the use of these devices to nonbiological particles [44].

    To overcome these limitations above, ideally one would like an architecture that combines the strong optical trapping force and low input optical power with the ability to manipulate nanoscopic matter precisely. Thus, in this paper, we propose a new optical trapping scheme via introducing a slot structure [51] into a 1D PC nanobeam cavity (1D-PCNC) to improve optical trapping capabilities. In this design, the slot structure possessing the advantage of excellent optical confinement can create strong optical intensities, gradients, and highly efficient optical trapping. First, a theoretical model is built to investigate the optical trapping force for a 10 nm radius PS nanoparticle in a symmetric mirror/microcavity/mirror system, and the analytical expression is obtained. Moreover, the theoretical analysis shows that the optical trapping force (F) is proportional to Tc·Q/V. Here, Tc represents the cavity transmissivity. Second, by using 3D-FEM (a commercial software package, COMSOL Multiphysics software) [52], the cavity trapping performances including achievable maximum trapping force, trapping stiffness, trapping stability, and trapping potential and threshold power for stable trapping are investigated. For trapping a PS nanoparticle of 10 nm radius within the cavity, the optical trapping force achieves a maximum value of 8.28 nN/mW at cavity transmissivity Tc=0.26, which is in accordance with the analysis results presented in previous work, denoting that the maximum optical trapping force occurs at the Tc0.25 [40,49]. Moreover, a trapping potential depth in this work as large as 1.15×105  kBTmW1 is obtained. Threshold power of only 0.087 μW is required for stable trapping, which is significantly decreased compared to previous PC cavity designs [3941,53].

    2. THEORY AND ANALYSIS

    In this work, the design of the theoretical analysis model is a symmetric mirror/microcavity/mirror system. The schematic is shown in Fig. 1(a). Here, the microcavity section serves as a photonic crystal cavity. The mirror sections on both sides of the microcavity section can be viewed as photonic crystal reflectors if the frequency of the incident light is within the photonic bandgap (PBG). In this system, light can be input from both sides and coupled into the microcavity through the coupling waveguide. The amplitudes of the input light on both sides are denoted by cin and din, respectively, as shown in Fig. 1(a). Here, we assume the inputs cin,din with the same frequency ωin. Otherwise, the case of inputs with different frequencies cannot be coherent and can be calculated individually. Note that there is no degeneracy between modes of the microcavity, and the difference of mode frequencies is much larger than the linewidth. Thus, we only take into account a single mode with frequency ω0, which is near ωin. The coupled-mode equation and input–output relation are given by where cout and dout represent the amplitude of output light from the left and right coupling waveguides, respectively. a is the amplitude of the microcavity mode. Δω=ωinω0 is the detuning between the frequency of the incident light and the cavity mode. κw is the coupling rate between the cavity and the dielectric waveguide, and κs is the intrinsic loss of the microcavity. The corresponding Q factor is Qw=ω0κw, Qs=ω0κs. The total Q factor can be expressed as 1Q=1Qw+1Qs [54].

    For convenience, we assume that the input light only comes from the left side, i.e., din=0 and the input power is Pin=|cin|2. Considering of the steady-state solution dadt=0, the amplitude of the cavity mode, and the output light can be expressed as

    (a) Schematic of the theoretical analysis model, which is a symmetric mirror/microcavity/mirror system. (b) Schematic of a nanoslotted-1D-PC nanobeam cavity for optical trapping. The structure is symmetric with respect to its center (blue dashed line). The trapped nanoparticle is shown within the slot. (c) Calculated Ey distribution (top view with z=0) of the fundamental resonant mode in the microcavity. (d) Ey profile along the centerline of the cavity in the x-direction. The units of the x/y-axis are micrometers (μm). (e) Optical trapping force F distribution profile and (f) trapping potential U distribution profile along the centerline of the cavity in the x-direction (solid line) and fitted Gaussian envelope function (dashed line), respectively, where a=560 nm, wnb=650 nm, h=220 nm, wslot=60 nm, rcenter=0.42a, rend=0.36a, Nt=20, and Nm=5 are chosen.

    Figure 1.(a) Schematic of the theoretical analysis model, which is a symmetric mirror/microcavity/mirror system. (b) Schematic of a nanoslotted-1D-PC nanobeam cavity for optical trapping. The structure is symmetric with respect to its center (blue dashed line). The trapped nanoparticle is shown within the slot. (c) Calculated Ey distribution (top view with z=0) of the fundamental resonant mode in the microcavity. (d) Ey profile along the centerline of the cavity in the x-direction. The units of the x/y-axis are micrometers (μm). (e) Optical trapping force F distribution profile and (f) trapping potential U distribution profile along the centerline of the cavity in the x-direction (solid line) and fitted Gaussian envelope function (dashed line), respectively, where a=560  nm, wnb=650  nm, h=220  nm, wslot=60  nm, rcenter=0.42a, rend=0.36a, Nt=20, and Nm=5 are chosen.

    The intracavity energy W=|a|2, reflectivity R=|cout|2|cin|2, and transmissivity Tc=|dout|2|cin|2 can be derived from Eq. (2) [54] as follows:

    It is found that when the detuning is much larger than the linewidth, i.e., |Δω|κw+κs, the light frequency falls into the PBG and the cavity mode cannot be excited efficiently, resulting in W and Tc almost being zero. When the cavity mode is on resonance, i.e., Δω=0, W and Tc achieve maximum values as follows:

    Here, we take a PS nanoparticle with radius r=10  nm as the trapped object. The optical trapping force (F) to a PS nanoparticle in the microcavity includes the gradient force and the scattering force. Furthermore, the scattering force is neglected due to the equilibrium of the standing wave mode. Thus, the gradient force can be calculated by regarding the particle as a dipole [3]:where P=αϵ0E represents the dipole moment of the particle. α=n21n2+24πr3 represents the polarizability of the sphere. By rewriting Eq. (5), the gradient force can be expressed as a function of intracavity energy and the relative field intensity distribution of that point, given as where Vc=Wϵ0Emax2 represents the mode volume of the cavity and f(r)2=E2(r)Emax2 represents the relative intensity distribution. Considering the variation of the field intensity within the particle, f(r)2 can be replaced by the average relative field intensity where Vp represents the volume of PS nanoparticles. As seen in Eq. (6), the optical trapping force is proportional to Tc·Q/V (i.e., FQTcV) for a nanoparticle at the fix point. Furthermore, the trapping potential U can be easily derived from Eq. (6), expressed as

    3. NANOSLOTTED-1D-PC NANOBEAM CAVITY DESIGN

    In this work, to validate the theoretical analysis in the above section, the basic structure of our design is a silicon-channel-waveguide-based nanoslotted-1D-PCNC. The schematic of the proposed nanoslotted-1D-PCNC is shown in Fig. 1(b). As seen, it is formed by introducing a nanoslotted structure in the middle of a 1D-PCNC, which consists of a single row of hole gratings embedded in a silicon nanobeam waveguide along horizontal x-axis, based on a silicon-on-insulator (SOI) platform with a 220 nm thick silicon device layer and a 2 μm thick buffer layer. The refractive indices of the silicon core layer and silica insulator layer are taken as nsi=3.46 and nsio2=1.45, respectively. The top cladding is assumed to be air (nair=1.0) in our numerical simulation [10,50]. To make the proposed device operate at the telecom wavelength range (1500  nm), the thickness and width of the silicon nanobeam waveguide are kept fixed as h=220  nm and wnb=650  nm, respectively. The periodicity of the hole gratings is a=560  nm to form a PC lattice. The structure is symmetric with respect to the center [the blue dashed line in Fig. 1(b)]. A basic 1D-PCNC cavity is formed by decreasing radii of the hole gratings while keeping the periodicity (a), slot width (wslot), and nanobeam waveguide width wnb unchanged. To achieve a high quality factor (Q) [55], (i) the hole gratings’ radii in the taper region of the proposed cavity are parabolically tapered from rcenter=0.42a in the center to rend=0.36a on both sides, i.e., ri=rcenter+(i1)2(rendrcenter)/(Nt1)2, where i increases from 1 to Nt and Nt represents the hole gratings’ number in the taper region of the cavity. Here, the radii of the hole gratings rcenter=0.42a and rend=0.36a are chosen from the numerical band diagram simulations [56]. (ii) The hole gratings’ radii in the mirror region of the proposed cavity are kept fixed as rj=rend=0.36a, where j increases from 1 to Nm and Nm represents the hole gratings’ number in the mirror region of the cavity. The design of the parabolically tapered hole structure is based on mode matching, which produces a significantly enhanced Q-factor and optical transmission through reductions in propagation losses and scattering that occur locally at transitions between the taper region and the mirror region of the cavity.

    Without loss of generality, TE-like cavity modes with electric field (E) mainly parallel to the x-y plane of the waveguide are considered in this work. Figures 1(c) and 1(d) show the top view of the major field (Ey) distribution profile of the fundamental resonant mode in the proposed cavity. It can be seen clearly that the maximum of the electric field occurs in the nanoslotted area at the center of the cavity, and the field distribution of fundamental resonant mode is highly concentrated. As shown in Fig. 1(e), the corresponding optical trapping forces (F) induced by the more concentrated mode will be stronger because of resonant enhancement and its sharp intensity gradient. Figure 1(f) shows the optical trapping potential (U) distribution profile along the centerline of the cavity in the x-direction. As seen, at the center of the cavity, the largest potential depth occurs. Thus, the nanoparticle will be stably trapped in this area due to the huge trapping potential depth of the cavity.

    Next, to investigate the interaction between the nanoparticle and the target resonant mode field distribution confined within the cavity, the proposed nanoslotted-1D-PCNCs with different slot widths (wslot), number (Nt) of hole gratings in the taper region, and number (Nm) of hole gratings in the mirror region are discussed in detail. Here, the trapped object is taken as a PS nanoparticle with radius r=10  nm and refractive index n=1.59 (for the wavelength near infrared). In the simulation, the trapped PS nanoparticle is placed at the vertical center with 50 nm separation between the cavity center corner (also the stable trapping position at x=0  nm, y=0  nm, and z=0  nm). That is, the trapped nanoparticle is centered at x=50  nm, y=0  nm, and z=0  nm. The optical trapping force is calculated by integrating the Maxwell stress tensor on the outer surface of the PS nanoparticle [28]. In this section, we consider the case when a waveguide mode is inserted into the cavity structure for one end of the coupling waveguide.

    First, we investigate the effect of different slot widths (wslot) on the cavity transmissivity (Tc), Q/V, trapping potential (U), and the induced optical trapping force (F, along the x-direction) on the PS nanoparticle, when wslot changes from wslot=0 to wslot=200  nm, while other parameters are kept fixed as wnb=650  nm, h=220  nm, a=560  nm, rcenter=0.42a, rend=0.36a, Nt=20, and Nm=10. The optical trapping force is normalized by input power in units of pN/mW. Figure 2(a) shows the cavity transmissivity (Tc) and Q/V as functions of different slot widths. As seen, with the slot width increased, the cavity transmissivity increases. In addition, when the slot width is between wslot=20  nm and wslot=60  nm, ultrahigh Q/V over 2.0×108 is achieved. Figure 2(b) shows the maximum optical trapping force (F) and trapping potential (U) on the 10 nm radius PS nanoparticle along the x-direction as a function of slot width. As seen, when the slot width is wslot=60  nm, an optical trapping force F as high as 2.66×103  pN/mW and a trapping potential U as high as 6.07×104  kBTmW1 can be achieved. Here we set T to be room temperature as 300 K (K=Kelvin). Figure 2(c) shows the electric field Ey distribution (top view) of the fundamental mode taken at the center of the silicon layer (z=0) as a function of slot width changed as wslot=0, 20, 40, 60, 80, 100, 150, and 200 nm, respectively. As seen, compared to the nonslotted cavity structure (wslot=0  nm), the proposed nanoslotted cavity structure can effectively confine light within the cavity, allowing combined hollow-core and liquid-core behavior and creating strong optical intensities and gradients. Here, we choose the slot width as wslot=60  nm in the following simulation.

    Influence of different slot widths on (a) cavity transmissivity Tc and Q/V, (b) maximum optical trapping force F and trapping potential U on a 10 nm radius PS nanoparticle, and (c) electric field Ey distributions (top view) taken at the center of the silicon layer (z=0) when wslot is changed from 0 to 200 nm and other parameters are kept fixed as wnb=650 nm, h=220 nm, a=560 nm, rcenter=0.42a, rend=0.36a, Nt=20, and Nm=10.

    Figure 2.Influence of different slot widths on (a) cavity transmissivity Tc and Q/V, (b) maximum optical trapping force F and trapping potential U on a 10 nm radius PS nanoparticle, and (c) electric field Ey distributions (top view) taken at the center of the silicon layer (z=0) when wslot is changed from 0 to 200 nm and other parameters are kept fixed as wnb=650  nm, h=220  nm, a=560  nm, rcenter=0.42a, rend=0.36a, Nt=20, and Nm=10.

    Second, from Eq. (6), we know that the optical trapping force is proportional to Tc·Q/V. That means that other than designing a suitable resonant mode with high Q/V, the efficient coupling between the input/output waveguide mode and the cavity resonant mode with high transmissivity (Tc) for efficient nanoparticle trapping needs to be considered. Thus, we change the period hole gratings’ number Nt (changed from Nt=5 to Nt=40) in the taper region and Nm (changed from Nm=0 to Nm=30) in the mirror region of the cavity [Fig. 1(b)], respectively, and investigate the effect of different values of Nt and Nm on the cavity transmissivity Tc, Q/V, trapping potential U, and the induced optical trapping force F (along the x-direction) on the 10 nm radius PS nanoparticle, when other parameters are kept fixed as wnb=650  nm, h=220  nm, wslot=60  nm, a=560  nm, rcenter=0.42a, and rend=0.36a, as shown in Fig. 3. As seen in Fig. 3(e), when Nt=20 and Nm=5, the maximum optical trapping force F on the 10 nm radius PS nanoparticle as high as 1.09×104  pN/mW can be achieved. A trapping potential U as high as 1.52×105  kBTmW1 can be achieved, which is enhanced by more than two orders of magnitude compared to the previous work [40,49,53]. When Nm is larger than 5 (Nm>5), enough for the nanoslotted photonic crystal lattice to provide the PBG effect, the proposed device can confine the resonant mode very well with ultrahigh Q/V over 2.0×108 [shown as Q/V versus Nm in Fig. 3(d)]. However, the good PBG effect reduces the coupling efficiency between the input/output waveguide mode and the cavity resonant mode [shown as Tc versus Nm in Fig. 3(d)], resulting in low cavity transmission. Thus, the optical trapping force induced by the weakly coupled resonance is rather small. On the contrary, when Nm is reduced and less than 5 (Nm<5), the cavity Q/V decreases because the confinement provided by the cavity PBG effect becomes weaker. For even smaller Nm, because the cavity resonant mode can no longer be supported by the insufficient PBG effect, resulting in the cavity Q/V decreased sharply and no resonance enhancing the optical trapping force, the induced optical trapping force becomes weaker again. As known from Section 2, the optical trapping force is proportional to the energy of the cavity. Thus, the maximum optical trapping force can be obtained in the case of a cavity with the largest energy. From Eq. (4), the energy stored in the cavity achieves its maximum when Qw=Qr for a given Qr, namely, Tc=0.25. As seen in Fig. 3(d), the simulation results show that when Nt=20 and Nm=5, the optical trapping force achieves the maximum value at the transmission of the cavity Tc=0.51, namely, the cavity transmission Tc=0.26 (near 0.25), which is in accordance with the theoretical analysis and the previous work [40,49]. Figures 3(c) and 3(f) display that the optical trapping force (F) varies with Tc·Q/V. As seen, the normalized optical trapping force (F) is proportional to Tc·Q/V, which further verifies the theoretical analysis in Section 2.

    Influence of different hole grating numbers Nt (changed from Nt=5 to Nt=40) in the taper region of the cavity on (a) cavity transmissivity Tc and Q/V, and (b) maximum optical trapping force F and trapping potential U on a 10 nm radius PS nanoparticle when Nm=10. Influence of different hole grating numbers Nm (changed from Nm=0 to Nm=30) in the mirror region of the cavity on (d) cavity transmissivity Tc and Q/V, and (e) maximum optical trapping force F and trapping potential U on a 10 nm radius PS nanoparticle when Nt=20. For both cases, other parameters are kept fixed as wnb=650 nm, h=220 nm, wslot=60 nm, a=560 nm, rcenter=0.42a, and rend=0.36a. (c), (f) Normalized optical trapping force F for the proposed cavity with different values of Tc·Q/V.

    Figure 3.Influence of different hole grating numbers Nt (changed from Nt=5 to Nt=40) in the taper region of the cavity on (a) cavity transmissivity Tc and Q/V, and (b) maximum optical trapping force F and trapping potential U on a 10 nm radius PS nanoparticle when Nm=10. Influence of different hole grating numbers Nm (changed from Nm=0 to Nm=30) in the mirror region of the cavity on (d) cavity transmissivity Tc and Q/V, and (e) maximum optical trapping force F and trapping potential U on a 10 nm radius PS nanoparticle when Nt=20. For both cases, other parameters are kept fixed as wnb=650  nm, h=220  nm, wslot=60  nm, a=560  nm, rcenter=0.42a, and rend=0.36a. (c), (f) Normalized optical trapping force F for the proposed cavity with different values of Tc·Q/V.

    4. NUMERICAL RESULTS AND DISCUSSION

    Herein, based on the simulation results and optimization process discussed in Section 3, a summary to show the structure parameters for the optimized nanoslotted-1D-PCNC are as follows: wnb=650  nm, h=220  nm, wslot=60  nm, a=560  nm, rcenter=0.42a, rend=0.36a, Nt=20, and Nm=5. To characterize the maximum optical trapping force in this system, the detailed numerical analysis and simulations performed here are based on the three-dimensional finite element method (3D-FEM). To determine the optical trapping force exerted on a PS nanoparticle, a virtual spherical surface enclosing the nanoparticle surface is constructed, and the electromagnetic field on this surface is calculated. Here, the size of the virtual surface is the same as the surface of the enclosed nanoparticle. Then, by evaluating the time-independent Maxwell stress tensor and integrating it over the closed surface that encloses the PS nanoparticle, the optical trapping force can be obtained. Here, the numerical technique consists of repeatedly calculating the optical trapping force while shifting the PS nanoparticle’s physical position along one of the main axes [Fig. 1(b)]. When canning the nanoparticle along the x- and z-axes, the virtual surface moves with the nanoparticle. Figures 4(a) and 4(b) display the plots of the normalized optical trapping force profile for a 10 nm radius PS nanoparticle that is displaced in x- and z-dimensions from the stable trapping position (namely, the cavity center with x=0, y=0, and z=0). As seen, the theoretical calculation results (solid blue line with plus sign) are consistent with the 3D-FEM numerical simulation results (dashed red line added with square). Figure 4(a) shows the trapping force (Fx, x component) for a 10 nm radius PS nanoparticle as it is located within the slot center (y=0 and z=0) and displaced along the length of the nanoslotted-1D-PCNC (x-axis). The zero x-axis value corresponds to the stable trapping position at the cavity center. As can be seen, because the nanoslotted-1D-PCNC structure is symmetric horizontally in the x-direction, the horizontal component optical force Fx exerted on the nanoparticle in the x-direction is mirror symmetric with respect to the cavity center. The trapping force Fx is negative for x>0, which means that when some perturbation floats the nanoparticle slightly away from the cavity center, the strength of the trapping force Fx increases progressively to pull the nanoparticle back toward the cavity center. As seen in Fig. 4(a), the trapping force (Fx) reaches a maximum at the point (x=50  nm) where the field gradient is strongest at the entrance between the nanoslot waveguide and the hole grating. By using 3D-FEM, the simulated maximum optical trapping force Fx for a 10 nm radius PS nanoparticle of 8.28×103  pN/mW is observed, which is two orders of magnitude higher than the maximum trapping force in the case of recent photonic crystal nanobeam cavities [4042,47,49] and several orders of magnitude higher than other optical trapping techniques based on nanoslotted waveguides [27,28]. In addition, when the nanoparticle floats away further in the x-direction (x>50  nm), the strength of the trapping force Fx declines along the x-direction as the nanoparticle position in the x-axis increases. That represents the characteristic of the evanescent field and indicates that the guided wave will lose its effect upon the nanoparticle. Figure 4(b) illustrates the vertical trapping forces (Fz, z component) exerted on a 10 nm radius PS nanoparticle for varying vertical positions along the height of the nanoslotted-1D-PCNC (z-axis) as it is located within the slot center (x=0 and y=0). Qualitatively, we note that (i) the vertical trapping force Fz is negative for z<0, which means nanoparticles that are located above the cavity center tend to exhibit a net downward force. This indicates that the optical gradient in the cavity tends to guide nanoparticles toward the middle of the device structure where the intensity is at its maximum. (ii) The vertical trapping force Fz attains its maximum value 6.56×103  pN/mW at z=110  nm corresponding to half of the thickness of the silicon device layer. (iii) Once the vertical trapping force Fz reaches its maximum value, it declines to zero as the nanoparticle position in z-axis increases, which represents the decay of the evanescent-wave-behaving region of the cavity structure.

    Numerical analysis of optical trapping forces for the proposed nanoslotted-1D-PCNC device. All theoretically computed and 3D-FEM simulated trapping forces listed are normalized by input power in units of pN/mW. Trapping force profiles of (a) Fx and (b) Fz for the PS nanoparticle as it is moved along the x-axis and z-axis of the device, respectively. In both (a) and (b), all calculations are done for a PS nanoparticle with a radius of 10 nm. Trapping potential distributions experienced by the PS nanoparticle along (c) the x-direction (ranging from x=−200 nm to x=200 nm) and (d) the z-direction (ranging from z=0 to z=200 nm).

    Figure 4.Numerical analysis of optical trapping forces for the proposed nanoslotted-1D-PCNC device. All theoretically computed and 3D-FEM simulated trapping forces listed are normalized by input power in units of pN/mW. Trapping force profiles of (a) Fx and (b) Fz for the PS nanoparticle as it is moved along the x-axis and z-axis of the device, respectively. In both (a) and (b), all calculations are done for a PS nanoparticle with a radius of 10 nm. Trapping potential distributions experienced by the PS nanoparticle along (c) the x-direction (ranging from x=200  nm to x=200  nm) and (d) the z-direction (ranging from z=0 to z=200  nm).

    By integrating the trapping force along the x-axis (ranging from x=200  nm to x=200  nm) with y=z=0  nm and along the z-axis (ranging from z=0 to z=200  nm) with x=y=0  nm, respectively, the corresponding potential U experienced by the PS nanoparticle can be obtained. Figures 4(c) and 4(d) show the corresponding potential distribution in the x- and z-direction, respectively. A criterion widely used for stable trapping requires depth of the potential energy (ΔU) larger than 10  kBT [3,40]. As seen in Figs. 4(c) and 4(d), based on 3D-FEM simulation results (red line), depths of the trapping potential (ΔU) along x- and z-directions as large as 1.15×105  kBTmW1 and 1.08×105  kBTmW1 are obtained, respectively, which are much deeper than the stable trapping requirement. Thus, the results manifest the trapping ability of the proposed slotted-1D-PCNC.

    From the calculated optical trapping force and trapping potential in Fig. 4, two parameters can commonly be extracted to describe optical trapping: one is the trapping stiffness (k), and the other is the trapping stability (Strap). In this system, for distances not far from the stable position, namely, the equilibrium point, the response of the optical trapping force is similar to a linear spring where the spring constant is equal to the trapping stiffness. Therefore, the trapping stiffness in the x-direction (kx) and the z-direction (kz) is the derivative of the restoring force Fx and Fz, respectively, with respect to the position perturbation around the equilibrium point, and can be described as follows [41]:

    Here, the other parameter of interest is the trapping stability (Strap), which leads to the average trapping time proportional to its exponential following a Kramers escaper process [57]. So the trapping stability (Strap) can be defined as the ratio of the potential energy depth (ΔU) to the available thermal energy [41]:

    Based on the optical trapping characteristics of the proposed nanoslotted-1D-PCNC design shown in Fig. 4, for a PS nanoparticle with a 10 nm radius, the calculated trapping stiffnesses in the x-direction and the z-direction are found to be kx=167.17  pN·nm1·  mW1 and kz=36.67  pN·nm1·mW1, respectively. The estimated trapping stiffness for this system is more than three orders of magnitude higher than those of the conventional photonic crystal nanobeam resonators [41,42] and more than two orders of magnitude higher than that of the recent slotted photonic crystal cavity [53]. In addition, as alluded to above, the trapping stability Strap is the ratio of the work energy required to remove the nanoparticle from the trap to the random thermal energy in the system. Based on Eq. (11), trapping stabilities as large as 1.15×105  mW1 are achieved in the proposed nanoslotted-1D-PCNC design. In order to achieve a stability factor equal to 10, which is generally considered sufficient to achieve stable trapping despite the presence of Brownian motion [3,53], the threshold power for stable trapping in this system is only 0.087 μW. A significant decrease of the optical power required for stable trapping can be achieved compared to previous designs, e.g., the power requirement for the stable trapping of a 25 nm radius PS nanoparticle in the slotted 2D-PC cavity (27 μW) [53], and the power requirement for the stable trapping of a 50 nm radius PS nanoparticle in the recent 1D-PC cavity with waist design (320 μW) [40]. Thus, the proposed optical trapping scheme based on nanoslotted-1D-PCNC in this work is a promising platform for achieving efficient trapping. In addition, we have summarized the trapping performances of different optical trapping schemes, as shown in Table 1. Here, although the performances of these different optical trapping systems shown in the table are not strict comparisons because they were performed with different size PS particles, we can find that the trapping performance of the proposed slotted-1D-PCNC is greatly improved compared with those of other optical trapping systems. The superposition of evanescent fields leads to an increase in the field intensity, as shown in Fig. 1(c). Thus, the optical force on a nanoparticle is enhanced by orders of magnitude, and the trapping stiffness is also significantly increased.

    Trapping SystemTrapping Particle Radius (nm)Trapping Force (pN/mW)Trapping Potentiala(kBT/mW)Trapping Stiffness (pN·nm1·mW1)Threshold Power (μW)References
    Solid waveguidePS, 2500.025[25]
    Slotted waveguidePS, 100.0071.41.31×1047.14×103[28]
    Ring resonatorPS, 2500.165.563.7×1041.8×103[29]
    2D-PCPS, 2503.8576.90.3130[39]
    1D-PCPS, 502.331.3320[40]
    PS, 504.2512.23×102196[41]
    PS, 100330[49]
    Slotted 2D-PCPS, 25463.77×1020.3427[53]
    Slotted 1D-PCNCPS, 108.28×1031.15×1051678.70×102Present work

    Table 1. Trapping Force, Trapping Potential, Trapping Stiffness, and Threshold Power of Various Optical Trapping Schemes

    So far, during the numerical results and discussion above, we have shown that a PS nanoparticle as small as 10 nm in radius can be stably trapped by the 1D-PCNC with the nanoslotted structure. In addition, it has already been outlined that for this type of 1D-PCNC device, the position and size of the nanoparticle within the slot/hole can affect the cavity resonant wavelength. By using 3D-FEM simulation, Fig. 5(a) displays the relation between the trapped single PS nanoparticle with different radii and the corresponding resonant peak wavelength of the transmission spectrum. Each of these trapped PS nanoparticles is positioned at the cavity center at x=0, y=0, and z=0. As seen, trapping of a single 25 nm radius PS nanoparticle causes a 0.6 nm redshift in peak wavelength, which is consistent with the results presented in previous designs [40,41,53]. Although the wavelength shift is small, it is still can be detected due to the narrow linewidth. Thus, the proposed nanoslotted-1D-PCNC device can be utilized to detect a single nanoparticle (e.g., dielectric and metallic nanoparticles) by observing the resonant peak wavelength shift in the transmission spectrum as demonstrated in Ref. [50]. Moreover, it also makes it possible to recognize the size of the trapped nanoparticle by the amount of peak shift. Figure 5(b) shows the magnitude of the maximum trapping force Fx in the x-direction as a function of the PS nanoparticle with different sizes/radii. Here, the nanoparticle position is maintained at 50  nm separated from the cavity center in the x-axis with x=50  nm, y=0 and z=0, as displayed in the inset in Fig. 5(a). As expected, PS nanoparticles of increasing radii experience stronger trapping forces in the nanoslotted-1D-PCNC.

    (a) 3D-FEM simulated the resonant peak wavelength of the transmission spectrum of the designed slotted 1D-PCNC when no nanoparticle is trapped and when a PS nanoparticle with a radius of 5, 10, 15, 20, or 25 nm is trapped at the cavity center with x=0, y=0, and z=0. (b) The graph shows the magnitude of the maximum trapping force Fx in the x-direction as a function of the PS nanoparticle with different sizes.

    Figure 5.(a) 3D-FEM simulated the resonant peak wavelength of the transmission spectrum of the designed slotted 1D-PCNC when no nanoparticle is trapped and when a PS nanoparticle with a radius of 5, 10, 15, 20, or 25 nm is trapped at the cavity center with x=0, y=0, and z=0. (b) The graph shows the magnitude of the maximum trapping force Fx in the x-direction as a function of the PS nanoparticle with different sizes.

    5. SUMMARY

    In summary, we have designed an ultracompact nanoslotted-1D-PCNC structure for nanoparticle manipulation and detection. In this structure, the advantages of both the 1D-PCNC (ultrahigh Q/V) and the nanoslotted waveguide (strong optical intensities and gradients) are combined to improve optical trapping capabilities so that much smaller nanoparticles can be manipulated. Numerical simulations indicate that the proposed nanoslotted-1D-PCNC can efficiently transport a PS nanoparticle with a diameter as small as 10 nm in a 60 nm slot. Here, excellent optical confinement and strong optical intensities and gradients provided by the device greatly enhance the optical trapping force exerted on the nanoparticle. For trapping a PS nanoparticle of 10 nm radius within the slot of the proposed device, a maximum optical trapping force as high as 8.28×103  pN/mW is obtained. In addition, the investigation of trapping potential shows that a threshold power lower than 0.1 μW is required for stable trapping, more than two orders of magnitude reduced compared to recent photonic-crystal-based optical trapping systems. Moreover, the numerical simulations show that the trapping of a single 25 nm radius PS nanoparticle causes a 0.6 nm redshift in resonant peak wavelength, which is consistent with the results presented in previous designs. Thus, the proposed device can be used for single nanoparticle detection by observing the resonant wavelength shift. Moreover, it also makes it possible to recognize nanoparticle size by analyzing the amount of wavelength shift. Therefore, the device presented in this work can potentially become a versatile platform for single nanoparticle, molecule, or virus manipulation and detection and other lab-on-a-chip applications in the future.

    Acknowledgment

    Acknowledgment. The authors thank Xiao-Chong Yu for fruitful discussions and help with simulations.

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    Daquan Yang, Fei Gao, Qi-Tao Cao, Chuan Wang, Yuefeng Ji, Yun-Feng Xiao. Single nanoparticle trapping based on on-chip nanoslotted nanobeam cavities[J]. Photonics Research, 2018, 6(2): 99
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