• Photonics Research
  • Vol. 5, Issue 3, 187 (2017)
Jinghuan Yang1、2, Quan Sun2, Han Yu2, Kosei Ueno2, Hiroaki Misawa2、3、5、*, and Qihuang Gong1、4、6、*
Author Affiliations
  • 1State Key Laboratory for Mesoscopic Physics and Department of Physics, Peking University, Beijing 100871, China
  • 2Research Institute for Electronic Science, Hokkaido University, Sapporo 001-0021, Japan
  • 3Department of Applied Chemistry, National Chiao Tung University, Hsinchu 30010, Taiwan
  • 4Collaborative Innovation Center of Quantum Matter, Beijing 100871, China
  • 5e-mail: misawa@es.hokudai.ac.jp
  • 6e-mail: qhgong@pku.edu.cn
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    DOI: 10.1364/PRJ.5.000187 Cite this Article Set citation alerts
    Jinghuan Yang, Quan Sun, Han Yu, Kosei Ueno, Hiroaki Misawa, Qihuang Gong. Spatial evolution of the near-field distribution on planar gold nanoparticles with the excitation wavelength across dipole and quadrupole modes[J]. Photonics Research, 2017, 5(3): 187 Copy Citation Text show less

    Abstract

    We investigate the superposition properties of the dipole and quadrupole plasmon modes in the near field both experimentally, by using photoemission electron microscopy (PEEM), and theoretically. In particular, the asymmetric near-field distributions on gold (Au) nanodisks and nanoblocks under oblique incidence with different polarizations are investigated in detail. The results of PEEM measurements show that the evolutions of the asymmetric near-field distributions are different between the excitation with s-polarized and p-polarized light. The experimental results can be reproduced very well by numerical simulations and interpreted as the superposition of the dipole and quadrupole modes with the help of analytic calculations. Moreover, we hypothesize that the electrons collected by PEEM are mainly from the plasmonic hot spots located at the plane in the interface between the Au particles and the substrate in the PEEM experiments.
    Eout=E0x^αE0[x^r33xr5(xx^+yy^+zz^)],(1)

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    α=a3ϵϵmϵ+2ϵm,(2)

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    Eout=E0x^+ikE0(xx^+zz^)αE0[x^r33xr5(xx^+yy^+zz^)]βE0[xx^+zz^r55zr7(x2x^+y2y^+xzz^)],(3)

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    β=a5ϵϵmϵ+3/2ϵm,(4)

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    Jinghuan Yang, Quan Sun, Han Yu, Kosei Ueno, Hiroaki Misawa, Qihuang Gong. Spatial evolution of the near-field distribution on planar gold nanoparticles with the excitation wavelength across dipole and quadrupole modes[J]. Photonics Research, 2017, 5(3): 187
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