• Infrared and Laser Engineering
  • Vol. 50, Issue 2, 20200342 (2021)
Qing Chang1, Hengyu Tan2、3, and Tianming Meng3
Author Affiliations
  • 1College of Media Engineering, Communication University of Zhejiang, Hangzhou 310018, China
  • 2Beijing Institute of Metrology, Beijing 100029, China
  • 3College of Electronic Engineering, Heilongjiang University, Harbin 150080, China
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    DOI: 10.3788/IRLA20200342 Cite this Article
    Qing Chang, Hengyu Tan, Tianming Meng. Nonlinear optics and ultrafast dynamics characteristics of CdTe/CdS quantum dots with different core sizes and shell thickness[J]. Infrared and Laser Engineering, 2021, 50(2): 20200342 Copy Citation Text show less
    Absorption spectra of the CdTe/CdS quantum dots
    Fig. 1. Absorption spectra of the CdTe/CdS quantum dots
    Open/closed aperture Z-scan normalized transmittance curves of water-soluble CdTe/CdS, S1-S2 quantum dots
    Fig. 2. Open/closed aperture Z-scan normalized transmittance curves of water-soluble CdTe/CdS, S1-S2 quantum dots
    Open/closed aperture Z-scan normalized transmittance curves of water-soluble CdTe/CdS, S3-S4 quantum dots
    Fig. 3. Open/closed aperture Z-scan normalized transmittance curves of water-soluble CdTe/CdS, S3-S4 quantum dots
    Open/closed aperture Z-scan normalized transmittance curves of water-soluble CdTe/CdS, S5-S6 quantum dots
    Fig. 4. Open/closed aperture Z-scan normalized transmittance curves of water-soluble CdTe/CdS, S5-S6 quantum dots
    Transient absorption spectra of water-soluble CdTe/ CdS, S1-S2 quantum dots
    Fig. 5. Transient absorption spectra of water-soluble CdTe/ CdS, S1-S2 quantum dots
    Transient absorption spectra of water-soluble CdTe/ CdS, S3-S4 quantum dots
    Fig. 6. Transient absorption spectra of water-soluble CdTe/ CdS, S3-S4 quantum dots
    Transient absorption spectra of water-soluble CdTe/ CdS, S5-S6 quantum dots
    Fig. 7. Transient absorption spectra of water-soluble CdTe/ CdS, S5-S6 quantum dots
    Ultrafast kinetic curves of water-soluble CdTe/CdS, S1-S2 quantum dots
    Fig. 8. Ultrafast kinetic curves of water-soluble CdTe/CdS, S1-S2 quantum dots
    Ultrafast kinetic curves of water-soluble CdTe/CdS, S3-S4 quantum dots
    Fig. 9. Ultrafast kinetic curves of water-soluble CdTe/CdS, S3-S4 quantum dots
    Ultrafast kinetic curves of water-soluble CdTe/CdS, S5-S6 quantum dots
    Fig. 10. Ultrafast kinetic curves of water-soluble CdTe/CdS, S5-S6 quantum dots
    Transient absorption spectrum of the solvent water
    Fig. 11. Transient absorption spectrum of the solvent water
    Sample numberQuantum dotsSize /nmCore colorCladding time
    S1CdTe/CdS-13.2Orange30 min
    S2CdTe/CdS-23.3orange1 h
    S3CdTe/CdS-33.0Yellow30 min
    S4CdTe/CdS-43.1Yellow1 h
    S5CdTe/CdS-52.6Green30 min
    S6CdTe/CdS-62.7Green1 h
    Table 1. Six kinds of the CdTe/CdS core-shell quantum dots
    Sample nameCore colorShellSize/nmβ/10-13 m·W-1n2/10−12esu χ3/10−14esu
    S1OrangeCdS-30 min3.24.391.423.85
    S2OrangeCdS-1 h3.35.011.494.12
    S3YellowCdS-30 min3.05.071.383.90
    S4YellowCdS-1 h3.15.291.854.92
    S5GreenCdS-30 min2.65.231.183.58
    S6GreenCdS-1 h2.76.421.734.92
    Table 2. Nonlinear optical parameters obtained from Z-scan measurement data for CdTe/CdS quantum dots
    Sample nameSizeτ-rise/ps τ1/ps τ2/ps
    S13.20.341.0617.81
    S23.30.331.9818.43
    S33.00.351.1313.79
    S43.10.592.1338.24
    S52.60.311.7412.77
    S62.70.321.7916.78
    Table 3. CdTe/CdS quantum dots fitting parameters
    Qing Chang, Hengyu Tan, Tianming Meng. Nonlinear optics and ultrafast dynamics characteristics of CdTe/CdS quantum dots with different core sizes and shell thickness[J]. Infrared and Laser Engineering, 2021, 50(2): 20200342
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