• Photonics Research
  • Vol. 6, Issue 6, 498 (2018)
Xiancui Su1, Baitao Zhang1,*, Yiran Wang1, Guanbai He1..., Guoru Li1, Na Lin1, Kejian Yang1, Jingliang He1,3 and Shande Liu2|Show fewer author(s)
Author Affiliations
  • 1State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, China
  • 2College of Electronics, Communication, and Physics, Shandong University of Science and Technology, Qingdao 266590, China
  • 3e-mail: jlhe@sdu.edu.cn
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    DOI: 10.1364/PRJ.6.000498 Cite this Article Set citation alerts
    Xiancui Su, Baitao Zhang, Yiran Wang, Guanbai He, Guoru Li, Na Lin, Kejian Yang, Jingliang He, Shande Liu, "Broadband rhenium disulfide optical modulator for solid-state lasers," Photonics Res. 6, 498 (2018) Copy Citation Text show less

    Abstract

    Rhenium disulfide (ReS2), a member of group VII transition metal dichalcogenides (TMDs), has attracted increasing attention because of its unique distorted 1T structure and electronic and optical properties, which are much different from those of group VI TMDs (MoS2, WS2, MoSe2, WSe2, etc.). It has been proved that bulk ReS2 behaves as a stack of electronically and vibrationally decoupled monolayers, which offers remarkable possibilities to prepare a monolayer ReS2 facilely and offers a novel platform to study photonic properties of TMDs. However, due to the large and layer-independent bandgap, the nonlinear optical properties of ReS2 from the visible to mid-infrared spectral range have not yet been investigated. Here, the band structure of ReS2 with the introduction of defects is simulated by the ab initio method, and the results indicate that the bandgap can be reduced from 1.38 to 0.54 eV with the introduction of defects in a suitable range. In the experiment, using a bulk ReS2 with suitable defects as the raw material, a few-layered broadband ReS2 saturable absorber (SA) is prepared by the liquid phase exfoliation method. Using the as-prepared ReS2 SA, passively Q-switched solid-state lasers at wavelengths of 0.64, 1.064, and 1.991 μm are in
    T=[1α0LIsIs+I0/(1+Z2/Z02)]/(1α0L),(1)

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    I=P¯outf·1+Roc1Roc·1πr2,(2)

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    Xiancui Su, Baitao Zhang, Yiran Wang, Guanbai He, Guoru Li, Na Lin, Kejian Yang, Jingliang He, Shande Liu, "Broadband rhenium disulfide optical modulator for solid-state lasers," Photonics Res. 6, 498 (2018)
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