1State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
2Hangzhou Institute for Advanced Study, University of Chinese Academy of Sciences, Hangzhou, Zhejiang 310024, China
3Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China
4School of Physical Science and Technology, Shanghai Tech University, Shanghai, 201210, China
Fig. 2. Wavelength tunability of perovskite nanomaterials. (a) By changing the ratio of iodine to bromine in MAPb(I1-xBrx)3, tuning of 786 to 544 nm can be achieved. Above is the absorption spectrum, below is an image of the nanocomposite[40]; (b) MAPbX3(X=Cl, Br, I) can be tuned to the emission wavelength from 390 to 790 nm in visible infrared by changing the ratio of hal
Fig. 3. Organo-inorganic hybrid perovskite WGM laser. (a) Near-infrared WGM laser for hexagonal and triangular perovskite MAPbI3-aXa nanocrystals[59]; (b) quadrilateral perovskite MAPbBr3 nanoplatelet with the increase of pump strength, the appearance of WGM laser and the optical excitation image of nanoplatelet above and below the threshold[60]; (c) WGM
Fig. 4. Different schemes of WGM mode laser. (a) WGM microcavity was formed by cross section of two crossed perovskite MAPbBr3 nanorods[64]; (b) tunable size of the perovskite CsPbX3 nano inorganic spheres WGM microcavity[65]; (c) WGM laser is realized by using silicon sphere as resonator[35]; (d) WGM mode laser is implemented
Fig. 5. Different schemes of WGM mode laser. (a) Schemes of inorganic perovskite CsPbBr3 quantum dots embedded silica sphere[72]; (b) CsPbBr3-SiO2 micro sphere into a diameter of 40 μm cylindrical tubes of luminous images, and the principle of laser WGM mode[72]; (c) CdS/CsPbBr3 shell/core structure[74]; (d) CsPb
Fig. 6. Perovskite nanowire laser. (a) Scheme of nanowire structure lasers[76-77]; (b) optical image of MAPbX3 perovskite nanowires with increased pump light intensity[44]; (c) with the increase of pumping intensity, intensity distribution of F-P mode perovskite MAPbIxCl3-x nanowires laser[
Fig. 7. All inorganic perovskite CsPbX3 nanowires. (a) Nanowire lasing image with different pump density[79]; (b) with the increase of excitation intensity, F-P mode laser appears on perovskite CsPbBr3 nanowires[79]; (c) nanowire laser can last for more than an hour (equivalent to 109 excitation cycles) with a fixed pulsed energy[
Fig. 8. Different schemes of F-P mode lasers. (a) F-P mode laser in all inorganic perovskite CsPbBr3 micron cube[86]; (b) SEM image of high-quality perovskite CsPbBr3 nano cubes using an improved low-temperature solution treatment method[87]; (c) schematic of the crystal structure and standing wave of the F-P cavity[87]; (d) inorganic
Fig. 10. Random lasers. (a) Random lasers using multiple scattering from a disordered medium[96]; (b) fluorescent images showing the pumping intensity, spatial distribution of perovskite MAPbI3 random lasers[97]; (c) emission spectrum diagrams below the pump threshold, close to the pump threshold, and above the pump threshold[97]; (d) TEM image o