• Photonics Research
  • Vol. 9, Issue 2, 151 (2021)
Jing Chen1, Chao Zhang1, Xiaolin Liu1, Lin Peng1, Jia Lin1、*, and Xianfeng Chen2、3
Author Affiliations
  • 1Department of Physics, Shanghai Key Laboratory of Materials Protection and Advanced Materials in Electric Power, Shanghai University of Electric Power, Shanghai 200090, China
  • 2State Key Laboratory of Advanced Optical Communication Systems and Networks, School of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240, China
  • 3Collaborative Innovation Center of Light Manipulation and Applications, Shandong Normal University, Jinan 250358, China
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    DOI: 10.1364/PRJ.410290 Cite this Article Set citation alerts
    Jing Chen, Chao Zhang, Xiaolin Liu, Lin Peng, Jia Lin, Xianfeng Chen. Carrier dynamic process in all-inorganic halide perovskites explored by photoluminescence spectra[J]. Photonics Research, 2021, 9(2): 151 Copy Citation Text show less

    Abstract

    Recently, all-inorganic halide perovskites have received enormous attention because of their excellent optoelectronic properties. Among them, the power conversion efficiency (PCE) of all-inorganic halide perovskite solar cells has made rapid progress in the last few years. However, understanding the intrinsic physical nature of halide perovskites, especially the dynamic process of photo-generated carriers, is a key for improving the PCE. In this review, we introduced and summarized the photoluminescence (PL) technique used to explore the carrier dynamic process in all-inorganic halide perovskites. Several physical models were proposed to investigate the dynamic parameters, i.e., recombination lifetime and diffusion length, by analyzing the steady-state PL as well as the time-resolved PL spectra. We also discussed the distinction of PL spectral behavior between bulk halide perovskite samples and those grown with transport layers due to the participation of different dominant dynamic paths. Finally, we briefly described some other optical techniques reported to study the relevant physical properties of all-inorganic halide perovskites.
    IPL(t)=A1e(tτ1)+A2e(tτ2)β.

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    Γ(T)=Γ0+σT+ΓLOeωLOkBT1,

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    I(T)=I01+AeEBkBT,

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    1τHeterojunction=1τPerovskite+1τCT,

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    ϕ=τHeterojunctionτCT.

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    n(x,t)t=D2n(x,t)x2k(t)n(x,t),

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    Jing Chen, Chao Zhang, Xiaolin Liu, Lin Peng, Jia Lin, Xianfeng Chen. Carrier dynamic process in all-inorganic halide perovskites explored by photoluminescence spectra[J]. Photonics Research, 2021, 9(2): 151
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