• Chinese Optics Letters
  • Vol. 21, Issue 5, 051402 (2023)
Qiang Fu1、2, Jing Qian1、2, Guande Wang1、2, and Quanzhong Zhao1、2、*
Author Affiliations
  • 1State Key Laboratory of High Field Laser Physics and CAS Center for Excellence in Ultra-intense Laser Science, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
  • 2University of Chinese Academy of Sciences, Beijing 100049, China
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    DOI: 10.3788/COL202321.051402 Cite this Article Set citation alerts
    Qiang Fu, Jing Qian, Guande Wang, Quanzhong Zhao. Heat accumulation effects in femtosecond laser-induced subwavelength periodic surface structures on silicon[J]. Chinese Optics Letters, 2023, 21(5): 051402 Copy Citation Text show less

    Abstract

    High-repetition rate femtosecond lasers are shown to drive heat accumulation processes that are attractive for femtosecond laser-induced subwavelength periodic surface structures on silicon. Femtosecond laser micromachining is no longer a nonthermal process, as long as the repetition rate reaches up to 100 kHz due to heat accumulation. Moreover, a higher repetition rate generates much better defined ripple structures on the silicon surface, based on the fact that accumulated heat raises lattice temperature to the melting point of silicon (1687 K), with more intense surface plasmons excited simultaneously. Comparison of the surface morphology on repetition rate and on the overlapping rate confirms that repetition rate and pulse overlapping rate are two competing factors that are responsible for the period of ripple structures. Ripple period drifts longer because of a higher repetition rate due to increasing electron density; however, the period of laser structured surface is significantly reduced with the pulse overlapping rate. The Maxwell–Garnett effect is confirmed to account for the ripple period-decreasing trend with the pulse overlapping rate.
    clTlt=kl2Tlz2,withCl=1.978+3.54×104Tl3.68Tl2[J/(cm3·K)]andkl=1585Tl1.23[W/(cm·K)],

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    Tl=m=1Amea2ωm2tsinωmz

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    Tl=AeB2t+C(B=ωklCl),

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    Λ=λ(λλsp+sinθ),

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    λsp=(λε1)1ε1+1ε(ω),

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    ε(ω)=εcωp2(ω2+γ2),

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    ωp=Neq2meε0,

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    Ne=2(mekBT2π)3/2Fξ(ηe),

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    Λ=λsp=λ1+1ε(ω).

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    εeff=ε1ε+2ε1+2f(εε1)ε+2ε1f(εε1),

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    Λ=λsp=(λεeff)1εeff+1ε.

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    Qiang Fu, Jing Qian, Guande Wang, Quanzhong Zhao. Heat accumulation effects in femtosecond laser-induced subwavelength periodic surface structures on silicon[J]. Chinese Optics Letters, 2023, 21(5): 051402
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