• Journal of Semiconductors
  • Vol. 41, Issue 5, 052205 (2020)
Boning Han1、2, Qingsong Shan1、2, Fengjuan Zhang1、2, Jizhong Song1、2、3, and Haibo Zeng1、2
Author Affiliations
  • 1School of Materials Science and Engineering, Nanjing University of Science and Technology, Nanjing 210094, China
  • 2MIIT Key Laboratory of Advanced Display Materials and Devices, Institute of Optoelectronics & Nanomaterials, Nanjing 210094, China
  • 3School of Physics and Engineering, Zhengzhou University, Zhengzhou 450052, China
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    DOI: 10.1088/1674-4926/41/5/052205 Cite this Article
    Boning Han, Qingsong Shan, Fengjuan Zhang, Jizhong Song, Haibo Zeng. Giant efficiency and color purity enhancement in multicolor inorganic perovskite light-emitting diodes via heating-assisted vacuum deposition[J]. Journal of Semiconductors, 2020, 41(5): 052205 Copy Citation Text show less

    Abstract

    Inorganic perovskites (CsPbX3 (X = I, Br, Cl)) have broad prospection in the field of high-definition displaying due to its excellent optoelectronic characteristics. The vacuum deposition process possesses advantages and competitiveness in the industrialized production. However, the performance of light emitting diodes (LEDs) based on vacuum-deposited is incredibly low. Herein, we proposed a heating-assisted vacuum deposition (HAVD) method to construct inorganic perovskite LEDs (PeLEDs) with enhanced performance. The roughness and crystallinity of perovskite film were improved by regulating the heating treatment of substrates. And the perovskite film exhibited largely rise in luminescence, with decreasing defect density. Consequently, with the optimized temperature, the green PeLEDs exhibited 100-fold improvement of external quantum efficiency (EQE) with the luminance of up to 11 941 cd/m2, and the full width at half-maximum (FWHM) of the electroluminescence (EL) spectra was decreased from 25 to 17 nm. At the same time, the red and blue PeLEDs also exhibited obvious enhancement in EQE and luminance by HAVD method, and both the FWHM of EL spectra dropped below 20 nm, exhibiting excellent high color purity. HAVD strategy has a huge potential to be a new commonly used method for low-cost fabrication of displays and lighting.
    $ {N_{\rm{defect}}} = 2\varepsilon {\varepsilon _0}{V_{\rm{TFL}}}/e{L^2}, $ (1)

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    $ J = \left( {{9 / 8}} \right)\varepsilon {\varepsilon _0}\mu \left( {{{{V^2}} / {{L^3}}}} \right). $ (2)

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    Boning Han, Qingsong Shan, Fengjuan Zhang, Jizhong Song, Haibo Zeng. Giant efficiency and color purity enhancement in multicolor inorganic perovskite light-emitting diodes via heating-assisted vacuum deposition[J]. Journal of Semiconductors, 2020, 41(5): 052205
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