• Chinese Journal of Lasers
  • Vol. 48, Issue 14, 1402019 (2021)
Qing Lin1、2、*, Naifei Ren2, Anran Song1, and Guangzhi Xia1
Author Affiliations
  • 1School of Mechanical and Electrical Engineering, Suqian College, Suqian, Jiangsu 223800, China
  • 2School of Mechanical Engineering, Jiangsu University, Zhenjiang, Jiangsu 212013, China
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    DOI: 10.3788/CJL202148.1402019 Cite this Article Set citation alerts
    Qing Lin, Naifei Ren, Anran Song, Guangzhi Xia. Mechanism of Femtosecond Laser-Induced Breakdown Mediated by Al/SiO2 Core/Shell Nanostructures[J]. Chinese Journal of Lasers, 2021, 48(14): 1402019 Copy Citation Text show less
    Al/SiO2 core/shell nanostructure and its meshing. (a) Mesh structure; (b) Al/SiO2 core-shell nanostructure
    Fig. 1. Al/SiO2 core/shell nanostructure and its meshing. (a) Mesh structure; (b) Al/SiO2 core-shell nanostructure
    Coupling flow chart
    Fig. 2. Coupling flow chart
    Calculation model of monomer
    Fig. 3. Calculation model of monomer
    Relative enhancement factor of electric field ξ for different morphology of Al/SiO2 core/shell nanoparticles in water. (a1)(a2) Monomer and its XZ cross section; (b1)(b2) dimer and its XZ cross section; (c1)(c2) trimer and its XZ cross section
    Fig. 4. Relative enhancement factor of electric field ξ for different morphology of Al/SiO2 core/shell nanoparticles in water. (a1)(a2) Monomer and its XZ cross section; (b1)(b2) dimer and its XZ cross section; (c1)(c2) trimer and its XZ cross section
    Proposed nanostructure and relative enhancement factor of electric field ξ at the center line of the nanostructure along Z-axis. (a) Proposed nanostructure; (b) relative enhancement factor of electric field ξ
    Fig. 5. Proposed nanostructure and relative enhancement factor of electric field ξ at the center line of the nanostructure along Z-axis. (a) Proposed nanostructure; (b) relative enhancement factor of electric field ξ
    Extinction cross-section for monomer, dimer and trimer of Al/SiO2 core/shell nanoparticles
    Fig. 6. Extinction cross-section for monomer, dimer and trimer of Al/SiO2 core/shell nanoparticles
    Evolution of plasma electron density for different morphology of Al/SiO2 core/shell nanoparticles. (a) Monomer; (b) dimer; (c) trimer
    Fig. 7. Evolution of plasma electron density for different morphology of Al/SiO2 core/shell nanoparticles. (a) Monomer; (b) dimer; (c) trimer
    Lattice temperature of different morphology of Al/SiO2 core/shell nanoparticles at corresponding laser breakdown fluence at t=1200 fs. (a) Monomer; (b) dimer; (c) trimer
    Fig. 8. Lattice temperature of different morphology of Al/SiO2 core/shell nanoparticles at corresponding laser breakdown fluence at t=1200 fs. (a) Monomer; (b) dimer; (c) trimer
    Evolution of lattice temperature of different morphology of Al/SiO2 core/shell nanoparticles
    Fig. 9. Evolution of lattice temperature of different morphology of Al/SiO2 core/shell nanoparticles
    Evolution of electron temperature of water plasma mediated by trimer
    Fig. 10. Evolution of electron temperature of water plasma mediated by trimer
    ParameterValueDescription
    λ /nm580Laser wavelength
    c0 /(m·s-1)3×108Speed of light in vacuum
    ωc0Angular frequency
    ε0 /(F·m-1)8.85×10-12Vacuum permittivity
    tp /fs300Laser pulse width [full width at half maximum (FWHM)]
    e /C1.6×10-19Electron charge
    mw /kg3×10-26Mass of water molecule
    ms /kg9.9765×10-26Mass of silica molecule
    me /kg9.10938291× 10-31Electron mass
    m's0.86meEffective silica electron mass[24]
    m'w0.5meEffective water electron mass[12,14]
    τ /fs1.6Mean free time between electron/molecule collisions[25]
    h- / ( J·s)1.0545718×10-34Reduced Planck constant
    Ew,gap /eV6.5Band gap energy of water[26]
    Es,gap /eV9Band gap energy of silica[27]
    ρw,bound /cm-36.68×1022Bound electron density of water[12]
    ρs,bound /cm-32.2×1022Bound electron density of silica[27]
    nw1.33Refractive index of water
    ns1.45Refractive index of silica
    ηrec /(cm3·s-1)2×10-9Empirical recombination rate[28]
    q0 /(W·m-2·K-1)133.4×106Thermal conductance at aluminum-silica interface[29]
    q1 /(W·m-2·K-1)1000×106Thermal conductance at silica-water interface[30]
    ρs /(kg·m-3)2203Density of silica
    ρw /(kg·m-3)1000Density of water
    cs /(J·kg-1·K-1)703Heat capacity of silica
    cw /(J·kg-1·K-1)4184Heat capacity of water
    ks /(W·m-1·K-1)1.38Thermal conductivity of silica
    kw /(W·m-1·K-1)0.61Thermal conductivity of water
    Table 1. Parameters used in multi-physical fields coupling model
    Qing Lin, Naifei Ren, Anran Song, Guangzhi Xia. Mechanism of Femtosecond Laser-Induced Breakdown Mediated by Al/SiO2 Core/Shell Nanostructures[J]. Chinese Journal of Lasers, 2021, 48(14): 1402019
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