• Chinese Optics Letters
  • Vol. 19, Issue 12, 123602 (2021)
Tianchen Zhao1, Qiang Ma1, Yajie Bian1, Yuyi Zhang1, Yiting Liu1, Xiaolei Zhang1、2、*, Botao Wu1、**, E Wu1、2, Shitao Lou1, and Qingyuan Jin1、***
Author Affiliations
  • 1State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200241, China
  • 2Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan 030006, China
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    DOI: 10.3788/COL202119.123602 Cite this Article Set citation alerts
    Tianchen Zhao, Qiang Ma, Yajie Bian, Yuyi Zhang, Yiting Liu, Xiaolei Zhang, Botao Wu, E Wu, Shitao Lou, Qingyuan Jin. Strong coupling with absorption and emission features of Ag@Au hollow nanoshells interacting with J-aggregated dye molecules[J]. Chinese Optics Letters, 2021, 19(12): 123602 Copy Citation Text show less

    Abstract

    We investigate the strong coupling from 5,5’,6,6’-tetrachloro-1,1’-diethyl-3,3’-di(4-sulfobutyl)-benzimidazolocarbocyanine (TDBC) molecules near pure nano-triangular Ag prisms or Ag@Au hollow nanoshells. When TDBC molecules are deposited on pure Ag nanoprisms or Ag@Au hollow nanoshells with the plasmonic resonance peak, matching very closely with the absorption band of TDBC J-aggregates, obvious Rabi splitting can be observed due to the strong coupling regime. Meanwhile, the photoluminescence intensity decreased with the increasing of the temperature, verifying the decreasing plasmon–exciton coupling interaction in the higher temperature. Our experimental results are coincident with the simulation results calculated by finite-difference time-domain method.
    g2>Γpl2+γ0216,

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    Tianchen Zhao, Qiang Ma, Yajie Bian, Yuyi Zhang, Yiting Liu, Xiaolei Zhang, Botao Wu, E Wu, Shitao Lou, Qingyuan Jin. Strong coupling with absorption and emission features of Ag@Au hollow nanoshells interacting with J-aggregated dye molecules[J]. Chinese Optics Letters, 2021, 19(12): 123602
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