Tuning exciton dynamics by the dielectric confinement effect in quasi-two-dimensional perovskites

Minghuan Cui; Chaochao Qin; Yuanzhi Jiang; Shichen Zhang; Changjiu Sun; Mingjian Yuan; Yonggang Yang; Yufang Liu

doi:10.1364/PRJ.500205

[1] N. Li, X. Niu, L. Li. Liquid medium annealing for fabricating durable perovskite solar cells with improved reproducibility. Science, 373, 561-567(2021).

[2] L. Wang, H. Zhou, J. Hu. A Eu³⁺ -Eu²⁺ ion redox shuttle imparts operational durability to Pb-I perovskite solar cells. Science, 363, 265-270(2019).

[3] Z. Liu, W. Qiu, X. Peng. Perovskite light-emitting diodes with EQE exceeding 28% through a synergetic dual-additive strategy for defect passivation and nanostructure regulation. Adv. Mater., 33, 2103268(2021).

[4] X. Liu, W. Xu, S. Bai. Metal halide perovskites for light-emitting diodes. Nat. Mater., 20, 10-21(2021).

[5] K. Lin, J. Xing, N. Q. Li. Perovskite light-emitting diodes with external quantum efficiency exceeding 20 percent. Nature, 562, 245-248(2018).

[6] C. Yu, N. Wang, T. He. Perovskite light-emitting diodes based on spontaneously formed submicrometre-scale structures. Nature, 562, 249-253(2018).

[7] Y. Hassan, J. H. Park, M. L. Crawford. Ligand-engineered bandgap stability in mixed-halide perovskite LEDs. Nature, 591, 72-77(2021).

[8] Y. Liu, J. Cui, K. Du. Efficient blue light-emitting diodes based on quantum-confined bromide perovskite nanostructures. Nat. Photonics, 13, 760-764(2019).

[9] G. Xing, N. Mathews, S. S. Lim. Low-temperature solution-processed wavelength-tunable perovskites for lasing. Nat. Mater., 13, 476-480(2014).

[10] Q. Zhang, Q. Shang, R. Su. Halide perovskite semiconductor lasers: materials, cavity design, and low threshold. Nano Lett., 21, 1903-1914(2021).

[11] S. C. Hou, M. K. Gangishetty, Q. M. Quan. Efficient blue and white perovskite light-emitting diodes via manganese doping. Joule, 2, 2421-2433(2018).

[12] M. K. Gangishetty, S. C. Hou, Q. M. Quan. Reducing architecture limitations for efficient blue perovskite light-emitting diodes. Adv. Mater., 30, 1706226(2018).

[13] M. Cui, C. Qin, Y. Jiang. Direct observation of competition between amplified spontaneous emission and Auger recombination in quasi-two-dimensional perovskites. J. Phys. Chem. Lett., 11, 5734-5745(2020).

[14] T. He, S. Li, Y. Jiang. Reduced-dimensional perovskite photovoltaics with homogeneous energy landscape. Nat. Commun., 11, 1672(2020).

[15] C. T. Zuo, A. Scully, D. Yak. Self-assembled 2D perovskite layers for efficient printable solar cells. Adv. Energy Mater., 9, 1803258(2019).

[16] M. J. Yuan, L. N. Quan, R. Comin. Perovskite energy funnels for efficient light-emitting diodes. Nat. Nanotechnol., 11, 872-877(2016).

[17] X. Gong, O. Voznyy, A. Jain. Electron-phonon interaction in efficient perovskite blue emitters. Nat. Mater., 17, 550-556(2018).

[18] H. H. Tsai, W. Y. Nie, J. C. Blancon. High-efficiency two-dimensional Ruddlesden–Popper perovskite solar cells. Nature, 536, 312-316(2016).

[19] Y. Zhang, J. Wen, Z. Xu. Effective phase-alignment for 2D halide perovskites incorporating symmetric diammonium ion for photovoltaics. Adv. Sci., 8, 2001433(2021).

[20] D. Ma, K. Lin, Y. Dong. Distribution control enables efficient reduced-dimensional perovskite LEDs. Nature, 599, 594-598(2021).

[21] X. Yang, X. Zhang, J. Deng. Efficient green light-emitting diodes based on quasi-two-dimensional composition and phase engineered perovskite with surface passivation. Nat. Commun., 9, 570(2018).

[22] R. L. Milot, R. J. Sutton, G. E. Eperon. Charge carrier dynamics in 2D hybrid metal halide perovskites. Nano Lett., 16, 7001-7007(2016).

[23] N. Wang, C. Lu, G. Rui. Perovskite light-emitting diodes based on solution-processed self-organized multiple quantum wells. Nat. Photonics, 10, 699-704(2016).

[24] C. Qin, T. Matsushima, W. Potscavage. Triplet management for efficient perovskite light-emitting diodes. Nat. Photonics, 14, 70-75(2020).

[25] M. Kumagai, T. Takagahara. Excitonic and nonlinear-optical properties of dielectric quantum-well structures. Phys. Rev. B, 40, 12359-12381(1989).

[26] G. Wu, R. Liang, Z. Zhang. 2D hybrid halide perovskites: structure, properties, and applications in solar cells. Small, 17, 2103514(2021).

[27] Y. Jiang, C. Qin, M. Cui. Spectra stable blue perovskite light-emitting diodes. Nat. Commun., 10, 1868(2019).

[28] C. Sun, Y. Jiang, M. Cui. High-performance large-area quasi-2D perovskite light-emitting diodes. Nat. Commun., 12, 2207(2021).

[29] Y. Tian, X. Qian, C. Qin. Modulating low-dimensional domains of self-assembling quasi-2D perovskites for efficient and spectra-stable blue light-emitting diodes. Chem. Eng. J, 415, 129088(2021).

[30] Y. Jin, Z. Wang, S. Yuan. Synergistic effect of dual ligands on stable blue quasi-2D perovskite light-emitting diodes. Adv. Funct. Mater., 30, 1908339(2020).

[31] J. T. Lin, C. C. Liao, C. S. Hsu. Harnessing dielectric confinement on tin perovskites to achieve emission quantum yield up to 21. J. Am. Chem. Soc., 141, 10324-10330(2019).

[32] Y. Jiang, M. Cui, S. Li. Reducing the impact of Auger recombination in quasi-2D perovskite light-emitting diodes. Nat. Commun., 12, 336(2021).

[33] B. Cheng, T. Y. Li, P. Maity. Extremely reduced dielectric confinement in two-dimensional hybrid perovskites with large polar organics. Commun. Phys., 1, 80(2018).

[34] J. Yin, P. Maity, R. Naphade. Tuning hot carrier cooling dynamics by dielectric confinement in two-dimensional hybrid perovskite crystals. ACS Nano, 13, 12621-12629(2019).

[35] R. Su, Z. Xu, J. Wu. Dielectric screening in perovskite photovoltaics. Nat. Commun., 12, 2479(2021).

[36] C. Song, H. Yang, F. Liu. Ultrafast femtosecond pressure modulation of structure and exciton kinetics in 2D halide perovskites for enhanced light response and stability. Nat. Commun., 12, 4879(2021).

[37] Q. Du, C. Zhu, Z. Yin. Stacking effects on electron−phonon coupling in layered hybrid perovskites via microstrain manipulation. ACS Nano, 14, 5806-5817(2020).

[38] W. Tao, C. Zhang, Q. Zhou. Momentarily trapped exciton polaron in two-dimensional lead halide perovskites. Nat. Commun., 12, 1400(2021).

[39] M. Cui, C. Qin, Z. Zhou. Tuning coherent phonon dynamics in two-dimensional phenylethylammonium lead bromide perovskites. Nano Res., 16, 3408-3414(2023).

[40] L. N. Quan, Y. Park, P. Guo. Vibrational relaxation dynamics in layered perovskite quantum wells. Proc. Natl. Acad. Sci. USA, 118, e2104425118(2021).

[41] C. Qin, M. Cui, D. Song. Ultrafast multiexciton Auger recombination of CdSeS. Acta Phys. Sin., 68, 107801(2019).

[42] K. Zhang, M. Niu, Z. Jiang. Multiple temporal-scale photocarrier dynamics induced by synergistic effects of fluorination and chlorination in highly efficient nonfullerene organic solar cells. Sol. RRL, 4, 1900552(2020).

[43] X. Hong, T. Ishihara, A. V. Nurmikko. Dielectric confinement effect on excitons in PbI₄-based layered semiconductors. Phys. Rev. B, 45, 6961-6964(1992).

[44] J. Hu, I. W. H. Oswald, S. J. Stuard. Synthetic control over orientational degeneracy of spacer cations enhances solar cell efficiency in two-dimensional perovskites. Nat. Commun., 10, 1276(2019).

[45] F. Thouin, D. A. Valverde-Chavez, C. Quarti. Phonon coherences reveal the polaronic character of excitons in two-dimensional lead halide perovskites. Nat. Mater., 18, 349-354(2019).

[46] J. Fu, M. Li, A. Solanki. Electronic states modulation by coherent optical phonons in 2D halide perovskites. Adv. Mater., 33, 2006233(2021).

[47] L. N. Quan, Y. Zhao, G. D. Pelayo. Tailoring the energy landscape in quasi-2D halide perovskites enables efficient green-light emission. Nano Lett., 17, 3701-3709(2017).

[48] R. Long, L. Jin, O. V. Prezhdo. Unravelling the effects of grain boundary and chemical doping on electron-hole recombination in CH₃NH₃PbI₃ perovskite by time-domain atomistic simulation. J. Am. Chem. Soc., 138, 3884-3890(2016).

[49] S. Martin, P. Samuel, G. Feliciano. Carrier lifetimes and polaronic mass enhancement in the hybrid halide perovskite CH₃NH₃PbI₃ from multiphonon Fröhlich coupling. Phys. Rev. Lett., 121, 086402(2018).

[50] D. Zhao, H. Hu, R. Haselsberger. Monitoring electron-phonon interactions in lead halide perovskites using time-resolved THz spectroscopy. ACS Nano, 13, 8826-8835(2019).

[51] H. Zhu, K. Miyata, Y. Fu. Screening in crystalline liquids protects energetic carriers in hybrid perovskites. Science, 353, 1409-1413(2016).

[52] K. Miyata, D. Meggiolaro, M. T. Tuan. Large polarons in lead halide perovskites. Sci. Adv., 3, e1701217(2017).

[53] Z. Guo, Y. Zhang, B. Wang. Promoting energy transfer via manipulation of crystallization kinetics of quasi-2D perovskites for efficient green light-emitting diodes. Adv. Mater., 33, 2102246(2021).

[54] C. Wang, G. Dai, J. Wang. Low-threshold blue quasi-2D perovskite laser through domain distribution control. Nano Lett., 22, 1338-1344(2022).

[55] X. Zhang, J. X. Shen, C. G. Van de Walle. Anomalous Auger recombination in PbSe. Phys. Rev. Lett., 125, 037401(2020).

[56] V. I. Klimov, A. A. Mikhailovsky, D. W. McBranch. Quantization of multiparticle Auger rates in semiconductor quantum dots. Science, 287, 1011-1013(2000).

[57] Y. Li, T. Ding, X. Luo. Biexciton Auger recombination in mono-dispersed, quantum-confined CsPbBr₃ perovskite nanocrystals obeys universal volume-scaling. Nano Res., 12, 619-623(2019).

[58] Y. Li, X. Luo, T. Ding. Size and halide dependent Auger recombination in lead halide perovskite nanocrystals. Angew. Chem. Int. Ed., 59, 14292-14295(2020).

[59] A. Hangleiter, R. Häcker. Enhancement of band-to-band Auger recombination by electron-hole correlations. Phys. Rev. Lett., 65, 215-218(1990).