We developed a hybrid structure photodetector combining one-dimensional (1D) inorganic GaAs nanowires and two-dimensional (2D) organic perovskite materials, which can achieve various performance enhancements using a relatively simple structure. Via the optical absorption enhancement of perovskite and the type-II energy band structure formed by the heterostructure, the responsivity and detectivity of the photodetector from ultraviolet (UV) to visible (Vis) wavelengths are significantly enhanced, reaching 75 A/W and 1.49×1011 Jones, respectively. The response time of the photodetector was significantly decreased by 3 orders, from 785 ms to 0.5 ms, and the dark current was further reduced to 237 fA. A photodetector was prepared with enhanced responsivity and ultrafast response time in the multiband region from the UV to Vis wavelength. To the best of our knowledge, this is the first time to combine inorganic III-V GaAs nanomaterials with organic perovskite materials, which verifies the effective combination of inorganic and organic materials in a mixed dimension. The excellent photoelectric performance of the perovskite/GaAs-nanowire hybrid structure photodetector makes it a potential candidate material for a wide range of photoelectric applications such as multiband photodetection.