
- Photonics Research
- Vol. 9, Issue 12, 2443 (2021)
Abstract
1. INTRODUCTION
Nonlinear optics in multimode optical fibers (MMFs) is an emerging research field, as it leads to new possibilities for the control of the spatial, temporal, and spectral properties of ultrashort light pulses [1]. Differently from the case of single-mode fibers, which are limited by their small transverse core size, large-area MMF permits for scaling up by orders of magnitude their energy transport capabilities. As a result, research in MMFs has attracted a growing interest for a variety of technologies, e.g., high-power fiber lasers [1], supercontinuum light sources [2], high-resolution biomedical imaging [3], and micromachining [4]. From a fundamental viewpoint, the high beam intensity that can be reached in MMFs has also led to unveiling different complex nonlinear phenomena [5,6].
The optical power transmission of MMFs is limited by different nonlinear effects, whose relative relevance strongly depends on the time scale of the propagating pulses. As well known, in the continuous-wave (cw) (or quasi-cw) regime, the power transmission limitation of optical fibers is set by Brillouin scattering [7]. When subnanosecond sources are employed, different nonlinear loss effects may become relevant. The electrons promoted from the valence to the conduction band by the absorption of pulses longer than tens of picoseconds interact with the atomic lattice, resulting in the heating of the fiber material. Injecting intense light pulses in optical fibers leads to thermally induced irreversible damage, such as fused silica melting and boiling [8,9]. Whenever the temperature reaches extreme values, typically above thousands of Kelvin, the fiber fuse phenomenon takes place [10]. On the other hand, when intense femtosecond pulses are injected into MMFs, the fiber may break down due to ionization phenomena: these typically occur when the laser intensity is above
Owing to the presence of a bandgap, ionization mechanisms in dielectric materials are triggered by multiphoton absorption (MPA) processes [13,14]. MPA plays a significant role even below the breakdown threshold, and it represents a major drawback for optical beam delivery, because it limits the efficiency of optical elements in the high-power regime. In fused silica, which is the main constituent of commercial MMFs, MPA may lead to nonlinear contributions to both the refractive index and the absorption coefficient, when operating at wavelengths between the visible and the mid-infrared range [15,16]. Because of the high intensities associated with the occurrence of MPA, its presence is generally neglected in a telecom context. Indeed, many photons need to be simultaneously absorbed to fill the pure silica bandgap (
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However, the presence of material defects, whose absorption band peaks at a few electronvolts, lowers the number of photons needed for the observation of MPA. For undoped core silica MMFs, the dominant defects, i.e., those with the highest oscillation strength, are the so-called non-bridging oxygen hole centers (NBOHCs) [18]. Recently, it has been shown that pulses at
In the particular case of graded-index fibers (GIFs), the germanium doping used to shape the core refractive index widens the range of defects, whose oscillation strength is comparable with that of NBOHCs. These defects are the Ge-related oxygen deficiency centers (Ge-ODCs), whose main characteristic is their blue-violet luminescence, and the paramagnetic Ge(1) and Ge(2) centers, which do not show any PL emission [18]. The PL of GIF defects permits directly visualizing the spatial self-imaging (SSI) phenomenon, the latter being the periodic replication of the electromagnetic field upon its propagation [20,21]. SSI is particularly studied in GIFs, since its period is remarkably short (a few hundreds micrometers), owing to the parabolic refractive index shape, which leads to equally spaced propagation constants for nondegenerate modes [22]. As a result, a laser beam propagating inside a GIF continuously widens and tightens its waist: correspondingly, PL generates a periodic array of light spots [23].
In this work, we investigate ultrashort pulse propagation in MMFs, in a power regime that is close but still below their breakdown value. Here MPA mechanisms turn out to be relevant, but no damages of the fiber material are induced yet. This permits us to carry out a detailed experimental characterization of optical nonlinear losses (NLs), which occur both in the normal and in the anomalous dispersion regimes of propagation. We first verify that thermal effects are not involved in determining such losses. Next, by comparing NL measurements of GIFs and step-index fibers (SIFs), we point out that SSI has a key role in enhancing those losses. We investigate the origin of NLs by comparing the wavelength dependence of the nonlinear fiber transmission properties with that of defects’ PL intensity. More specifically, we study the fiber power transmission properties when varying the fiber length, as well as the input beam wavelength and pulse width. In the femtosecond regime, we found that MPA, which is responsible for PL, is one of the main contributors to NLs. To reproduce our observations, we introduce an analytical model, where an effective N-photon absorption term is added to the propagation equation. A value of
2. EXPERIMENTS
The experimental setup to study NL phenomena in MMFs is shown in Fig. 1. It consists of an ultrashort laser system, involving a hybrid optical parametric amplifier (OPA) of white-light continuum (Lightconversion ORPHEUS-F), pumped by a femtosecond Yb-based laser (Lightconversion PHAROS-SP-HP), generating pulses at 10 to 100 kHz repetition rate and
Figure 1.Experimental setup to characterize the NL of MMFs. In the inset, we show a microscope image of the scattered PL in correspondence of the self-imaging points of a 50/125 GIF. The white scale bar is 1 mm long.
A. Optical Nonlinear Losses
Optical NLs consist of the transmission decrease when high-power pulses are injected into the fiber. This is shown in Fig. 2(a), where we report the input energy (
Figure 2.(a) Dependence of output pulse energy versus the input energy, at
In Figs. 2(c) and 2(d), we report the output spectra corresponding to the data of Fig. 2(a). As we can see, the two dispersion regimes lead to strongly different behaviors. At
By comparing Figs. 2(a), 2(c), and 2(d), we found that, in both dispersion regimes, MPA properties are remarkably similar, in spite of the profound differences in spectral and temporal dynamics. This permits us to justify the derivation, in Section 3, of a simple model for describing the effects of MPA on beam propagation, which only takes into account spatial effects.
B. Fiber Breakdown
When operating at pulse intensities of the same order of magnitude as the laser-induced breakdown threshold, one naturally wonders whether irreversible processes may occur in the fiber. We verified that our experiments can be repeated several times without observing any alteration of the fiber properties. However, we investigate the possible role played by thermal effects. These deal with the vibration of the atomic lattice (phonons), whose motion is much slower if compared to the laser pulsewidth. Therefore, thermal phenomena necessarily must depend on the beam average power, so that their effect of the optical transmission can be experimentally investigated by varying the laser repetition rate. We checked that the fiber output power linearly scales with the laser repetition rate at peak powers in both the linear loss and the NL regimes (Fig. 3). This proves that thermal effects are negligible in our experiments. We also monitored the output transmission during the whole experiment, without noticing appreciable variations. On the other hand, we repeated the experiments with longer pulses that are above 1 ps in temporal duration. Differently from the femtosecond regime, at the same values of peak power, we observed that the fiber transmission slowly but significantly drops in time. In particular, we monitored the transmission for several minutes, observing its progressive reduction (not shown), which is a sign of fiber breakdown. The input tip of the fiber was imaged by the optical microscope working in cross-polarizer configuration in order to maximize the scattering from damages (see the inset of Fig. 3). As can be seen, irreversible modifications of the sample were formed close to the input facet of the fiber, in proximity of the self-focusing point.
Figure 3.Output average power versus the laser repetition rate, for 0.8 MW (linear loss regime) or 1.9 MW (NL regime) of input power. The laser wavelength and pulse duration were set to 1030 nm and 174 fs, respectively. The inset shows a microscope image of the input tip of a 50/125 GIF, after picosecond laser pulses with power right above the breakdown threshold were injected for a few minutes.
C. Role of Spatial Self-Imaging
The results shown so far exclude the role of dispersion and thermal effects on the physical mechanism responsible for the femtosecond NL. Here we show that the spatial evolution of the beam inside the fiber is the key element for activating the nonlinear optical attenuation. For doing so, we compare the nonlinear transmission properties of MMFs with the same core/cladding size, with (GIF) or without (SIF) SSI. As a result of MPA, one observes the upconversion PL of silica defects, which, thanks to its typical violet color, helps track the spatial dynamics of the beam inside the MMFs. This permits us to visualize the different beam evolutions that take place inside the SIF and the GIF. Optical beams propagating in an SIF experience a single self-focusing point at the very beginning of the fiber [see the digital microscope image of PL in Figs. 4(a) and 4(c)]. The resulting high intensity leads to MPA, so that most of the beam energy is lost over the first few millimeters of propagation. Conversely, in a GIF the beam diameter periodically oscillates in space, owing to SSI [1]. The associated spatial beam breathing produces several minima for the beam diameter, where MPA may lead to NL. As a result, as shown in Figs. 4(b) and 4(d), PL appears as an array of equally spaced emitting points [23]. The different beam dynamics for the two types of MMF have direct consequence on power transmission measurements. In Fig. 4(e), we report the optical transmission as a function of the input pulse energy, for input pulse durations of either 174 fs or 7.9 ps, with
Figure 4.(a) and (b) Microscope images of the (a) SIF and (b) GIF when the defects’ PL is excited by MPA of a 2 MW input peak power laser beam. (c), (d) Same as (a), (b), with the room light switched off. The white bar is 1 mm long. (e) Comparison between the two MMFs normalized transmission, versus input pulse energy, for a pulse duration of 174 fs (circle markers, solid lines) or 7.9 ps (square markers, dashed lines).
D. Spectral Analysis
With the aim of investigating the physical origin of MPA, we studied how both PL and fiber transmission vary with the source wavelength. As depicted in the setup of Fig. 1, we collected the PL signal into a VIS-IR spectrometer. In Figs. 5(a) and 5(b) we show measured scattered spectra and input spectra, respectively, for a laser peak power of 2.5 MW, and wavelengths varying between 680 and 900 nm. Besides the spectral broadening of the pump, observed spectra display the characteristic NBOHC and the Ge-ODC PL peaks, occurring at 650 and 400 nm, respectively. Following the same method as in Ref. [19], we suppose a power-law linking the Ge-ODC PL intensity (
Figure 5.(a) Side-scattered spectra for different source wavelengths at
Next, we compared the analysis of the wavelength dependence of side-scattered spectra with that of fiber transmission measurements. As shown by Fig. 5(d), NL was observed at all source wavelengths. Nonetheless, differently from the PL related curves of Fig. 5(c), the transmission curves are not sorted with respect to the input wavelength. This indicates that Ge-ODC and NBOHC absorption is not the only mechanism that is responsible for NLs. For a clearer comparison, in Fig. 5(e) we simultaneously plot the wavelength dependence of both
E. Macroscopic Spatial Evolution
In order to track the spatial evolution of PL along the beam propagation, we placed the spectrometer and the lens on a translation stage, which allows for shifting them solidly. In Fig. 6(a) we show the longitudinal evolution of the side-scattered light spectrum, over the first centimeter of a GIF, for 2.5 MW of input peak power. Besides the pump at 1030 nm, three additional main peaks appear: the third harmonic (TH) at 343 nm and two PL peaks at 400 and 650 nm, respectively. The resulting collected spectra were postprocessed in order to determine the evolution of the spectral energy associated with each peak. Figure 6(b) shows that the energy of PL peaks significantly drops over less than 1 cm of fiber. On the other hand, our measurements (not shown here) reveal that the TH (and the pump) energy is only damped over several centimeters (or several tens of centimeters). The observed decrease of the PL is associated with a drop of the peak intensity of the beam. However, the drop of PL intensity does not necessarily prove a loss of the beam energy. For example, an intensity decrease may be due to a temporal broadening of the pulses, to modal walk-off, or to an increase of the effective area of the beam. However, the observed rapid damping of light side-scattered by the pump indicates that, even if present, these contributions are negligible in our case [i.e., for a propagation distance of the order of 1 cm, as in Fig. 2(a)].
Figure 6.(a) Side-scattering spectrum, obtained when varying the slit position. (b) Integral of the spectral peaks in (a). Solid lines are a guide for the eye. (c) Cutback experiment from 10 cm to 1.5 cm of fiber length. The
In order to verify that indeed MPA processes are responsible for the observed PL signal drop of Fig. 6(b), we performed a cut-back experiment by progressively reducing the GIF length from 10 cm down to 1.5 cm, while keeping the input coupling conditions unchanged. The measured transmission as a function of
3. ANALYTICAL MODEL
Let us consider the beam spatial dynamics under the slowly varying envelope approximation, treating time as a parameter, analogously to the variational approach proposed by Karlsson et. al. [25]. In order to take into account the experimental NL, we added to the index grading and the Kerr nonlinearity, an effective
Figure 7.(a) Detail of the beam size minimum, for different values of
In an MPA process, the energy loss strongly depends on the beam waist through its intensity. At points of maximum intensity, the MPA contribution becomes most relevant. Even though the absorption coefficient is small, the intensity locally reaches such high values that the NL term in Eq. (3) is no longer negligible. This results in a series of stepwise drops of the transmission curve at points of SSI-induced beam focusing as shown in Fig. 7(c).
One may object that
As a last result, we fitted the experimental data of the cutback measurements in Fig. 6(c) with our analytical model (see Appendix B for details). As shown in Fig. 8, we obtained a good quantitative agreement: the fitting function interpolates well experimental data for all values of
Figure 8.Fit of the cutback experimental data in Fig.
4. CONCLUSION
We experimentally characterized nonlinear optical losses in MMFs when operating slightly below the breakdown power threshold. In this regime, MPA mechanisms play a significant role, and may strongly affect the dynamics of the propagating beam. For example, in the anomalous dispersion regime, it has been shown that MPA clamps the beam output energy, thus suppressing the Raman soliton self-frequency shift [24]. In this work, based on the observed close similarity between nonlinear power transmission properties of MMFs in both the normal and the anomalous dispersion regimes, we carried out a detailed investigation of the spatial beam dynamics. Specifically, we revealed that SSI has a key role in enhancing NL. Therefore, MPA effects are remarkably higher in GIFs than in SIFs. By comparing side-scattering and transmission measurements, we could infer that the observed NL cannot be entirely ascribed to the MPA, which is associated with defects’ PL. Although all of the different sources of NL could not be directly identified, we demonstrated that the observed nonlinear transmission drop could be quantitatively well reproduced by introducing an effective N-photon absorption term in the propagation equation. Namely, we found that
Acknowledgment
Acknowledgment. We acknowledge support from the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation program, and the Italian Ministry of University and Research.
APPENDIX A: THEORETICAL MODEL
In this appendix we show the step-by-step derivation of Eq. (
APPENDIX B: CUTBACK EXPERIMENT FITTING
Equation (
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