• Matter and Radiation at Extremes
  • Vol. 5, Issue 6, 064201 (2020)
F. B. Rosmej1、2、3、4、a), V. A. Astapenko3, V. S. Lisitsa3、4、5, and L. A. Vainshtein6
Author Affiliations
  • 1Sorbonne University, Faculty of Science and Engineering, UMR 7605, Case 128, 4 Place Jussieu, F-75252 Paris Cedex 05, France
  • 2LULI, Ecole Polytechnique, CNRS-CEA, Physique Atomique dans les Plasmas Denses (PAPD), Route de Saclay, F-91128 Palaiseau Cedex, France
  • 3Moscow Institute of Physics and Technology MIPT (National Research University), Dolgoprudnyi 141700, Russia
  • 4National Research Nuclear University—MEPhI, Department of Plasma Physics, Moscow 115409, Russia
  • 5National Research Center “Kurchatov Institute”, Moscow, Russia
  • 6P. N. Lebedev Physical Institute of the Russian Academy of Sciences, Moscow 119991, Russia
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    DOI: 10.1063/5.0014158 Cite this Article
    F. B. Rosmej, V. A. Astapenko, V. S. Lisitsa, L. A. Vainshtein. Dielectronic recombination in non-LTE plasmas[J]. Matter and Radiation at Extremes, 2020, 5(6): 064201 Copy Citation Text show less
    Energy-level diagram of the He-like autoionizing levels 2l2l′ and their associated radiative decays, so-called Lyα satellites. After radiative decay, the singly excited states 1s2l1,3L are formed, from which further radiative decay proceeds (e.g., the resonance and intercombination lines W and Y, respectively). Also indicated are the Li-like autoionizing levels 1s2l2l′.
    Fig. 1. Energy-level diagram of the He-like autoionizing levels 2l2l′ and their associated radiative decays, so-called Lyα satellites. After radiative decay, the singly excited states 1s2l1,3L are formed, from which further radiative decay proceeds (e.g., the resonance and intercombination lines W and Y, respectively). Also indicated are the Li-like autoionizing levels 1s2l2l′.
    MARIA simulations of dielectronic satellite emission near Lyα of H-like Mg ions for different values of the electron density at kTe = 100 eV. The red arrows indicate the rises in intensity of particular satellite transitions with increasing density. Satellites indicated in blue have effective negative screening due to strong angular-momentum coupling effects.
    Fig. 2. MARIA simulations of dielectronic satellite emission near Lyα of H-like Mg ions for different values of the electron density at kTe = 100 eV. The red arrows indicate the rises in intensity of particular satellite transitions with increasing density. Satellites indicated in blue have effective negative screening due to strong angular-momentum coupling effects.
    Comparison of the l-averaged statistical approach with the Burgess and quantum level-by-level calculations for the Ni-like sequence 3s23p63d10 of Xe26+ and Au51+.
    Fig. 3. Comparison of the l-averaged statistical approach with the Burgess and quantum level-by-level calculations for the Ni-like sequence 3s23p63d10 of Xe26+ and Au51+.
    Comparison of the l-averaged statistical approach with the Burgess and quantum level-by-level calculations for the Sr-like sequence 4s24p64d2 of W36+ and the Zn-like sequence 4s2 of tungsten W44+.
    Fig. 4. Comparison of the l-averaged statistical approach with the Burgess and quantum level-by-level calculations for the Sr-like sequence 4s24p64d2 of W36+ and the Zn-like sequence 4s2 of tungsten W44+.
    Element1s22lnl′: α0 = 1s22sα = 1s22p
    Bd(1- channel)Bd(multichannel)Bd(Burgess)
    Be8.09 × 10−51.34 × 10−4
    C5.18 × 10−57.99 × 10−5
    Mg1.34 × 10−51.94 × 10−5
    Ar6.87 × 10−68.65 × 10−6
    Fe4.02 × 10−64.88 × 10−6
    Mo3.11 × 10−63.87 × 10−6
    1s23lnl′: α0 = 1s22sα = 1s23p
    Be3.44 × 10−51.97 × 10−62.88 × 10−5
    C6.45 × 10−56.61 × 10−66.98 × 10−5
    Mg6.43 × 10−52.57 × 10−56.96 × 10−5
    Ar4.55 × 10−52.42 × 10−55.15 × 10−5
    Fe2.61 × 10−51.57 × 10−53.54 × 10−5
    Mo8.61 × 10−66.48 × 10−61.89 × 10−5
    1s24lnl′: α0 = 1s22sα = 1s24p
    Be1.60 × 10−53.47 × 10−71.10 × 10−5
    C2.52 × 10−53.39 × 10−72.23 × 10−5
    Mg2.06 × 10−51.30 × 10−61.87 × 10−5
    Ar1.29 × 10−52.05 × 10−61.27 × 10−5
    Fe6.54 × 10−62.00 × 10−68.01 × 10−6
    Mo1.87 × 10−61.17 × 10−63.82 × 10−6
    Table 1. Bd factors according to Eqs. (3.20) and (3.21) for DR into Li-like ions originating from the 1s2nlnl′ autoionizing levels, with Z = Zn − 2, m = 1, and l0 = 0. The numerical data show single- and multichannel approximations as well as the corresponding factors according to the Burgess approach (note that the different numerical coefficients and the oscillator strength in the original Burgess formula [Eq. (3.10)] compared with Eq. (3.20) have been included in the value for Bd(Burgess) to facilitate comparison of the different methods).
    2lnl′: α0 = 1sα = 2p3lnl′: α0 = 1sα = 3p
    ElementBdχdBdχd
    He3.12 × 10−40.7445.48 × 10−60.888
    Li3.72 × 10−40.7366.41 × 10−60.887
    Be3.67 × 10−40.7276.53 × 10−60.885
    B3.42 × 10−40.7186.47 × 10−60.883
    C3.13 × 10−40.7096.32 × 10−60.881
    N2.85 × 10−40.7006.31 × 10−60.879
    O2.58 × 10−40.6915.92 × 10−60.877
    F2.33 × 10−40.6825.70 × 10−60.874
    Ne2.11 × 10−40.6735.48 × 10−60.872
    Na1.90 × 10−40.6655.26 × 10−60.870
    Mg1.72 × 10−40.6575.04 × 10−60.868
    Al1.56 × 10−40.6494.84 × 10−60.866
    Si1.41 × 10−40.6424.63 × 10−60.863
    P1.27 × 10−40.6364.43 × 10−60.861
    S1.15 × 10−40.6304.24 × 10−60.859
    Cl1.05 × 10−40.6244.05 × 10−60.857
    Ar9.50 × 10−50.6203.87 × 10−60.856
    K8.61 × 10−50.6163.69 × 10−60.854
    C7.82 × 10−50.6123.52 × 10−60.852
    Sc7.09 × 10−50.6093.35 × 10−60.851
    Ti6.45 × 10−50.6063.19 × 10−60.849
    V5.85 × 10−50.6043.04 × 10−60.848
    Cr5.33 × 10−50.6022.89 × 10−60.847
    Mn4.85 × 10−50.6012.74 × 10−60.846
    Fe4.42 × 10−50.5992.60 × 10−60.845
    Co4.03 × 10−50.5982.47 × 10−60.844
    Ni3.68 × 10−50.5982.34 × 10−60.843
    Cu3.37 × 10−50.5972.22 × 10−60.842
    Zn3.08 × 10−50.5972.10 × 10−60.842
    Ga2.83 × 10−50.5961.99 × 10−60.842
    Ge2.60 × 10−50.5961.88 × 10−60.841
    As2.39 × 10−50.5961.78 × 10−60.841
    Se2.20 × 10−50.5961.68 × 10−60.841
    Br2.03 × 10−50.5961.59 × 10−60.841
    Kr1.88 × 10−50.5961.50 × 10−60.841
    Rb1.74 × 10−50.5971.42 × 10−60.841
    Sr1.61 × 10−50.5971.34 × 10−60.842
    Y1.50 × 10−50.5971.27 × 10−60.842
    Zr1.39 × 10−50.5981.20 × 10−60.842
    Nb1.30 × 10−50.5991.13 × 10−60.843
    Mo1.21 × 10−50.5991.07 × 10−60.843
    Table 2. Fitting coefficients according to Eqs. (3.20) and (3.21) for DR into H-like ions originating from the 2lnl′ and 3lnl′ autoionizing levels, with Z = Zn, m = 1, and l0 = 0. The numerical data include corrections for multiple decay channels (two channels for 2lnl′ and four channels for 3lnl′).
    1s2lnl′: α0 = 1s2α = 1s2p1s3lnl′: α0 = 1s2α = 1s3p
    ElementBdχdBdχd
    Li3.39 × 10−51.111.57 × 10−61.27
    Be9.94 × 10−50.9612.12 × 10−61.14
    B1.53 × 10−40.8912.51 × 10−61.07
    C1.93 × 10−40.8482.98 × 10−61.03
    N2.17 × 10−40.8183.40 × 10−61.00
    O2.34 × 10−40.7953.92 × 10−60.983
    F2.17 × 10−40.7754.23 × 10−60.967
    Ne2.05 × 10−40.7574.50 × 10−60.956
    Na1.88 × 10−40.7404.56 × 10−60.945
    Mg1.72 × 10−40.7264.54 × 10−60.937
    Al1.57 × 10−40.7134.47 × 10−60.929
    Si1.43 × 10−40.7014.36 × 10−60.922
    P1.30 × 10−40.6904.22 × 10−60.916
    S1.18 × 10−40.6814.07 × 10−60.910
    Cl1.07 × 10−40.6723.92 × 10−60.905
    Ar9.72 × 10−50.6643.76 × 10−60.901
    K8.83 × 10−50.6583.61 × 10−60.897
    C8.02 × 10−50.6523.45 × 10−60.893
    Sc7.28 × 10−50.6473.30 × 10−60.889
    Ti6.62 × 10−50.6423.15 × 10−60.886
    V6.02 × 10−50.6383.01 × 10−60.883
    Cr5.47 × 10−50.6352.87 × 10−60.880
    Mn4.98 × 10−50.6322.73 × 10−60.877
    Fe4.54 × 10−50.6292.60 × 10−60.875
    Co4.14 × 10−50.6272.47 × 10−60.873
    Ni3.78 × 10−50.6252.35 × 10−60.871
    Cu3.46 × 10−50.6232.23 × 10−60.869
    Zn3.16 × 10−50.6222.11 × 10−60.868
    Ga2.90 × 10−50.6202.00 × 10−60.867
    Ge2.67 × 10−50.6191.90 × 10−60.865
    As2.45 × 10−50.6191.80 × 10−60.864
    Se2.26 × 10−50.6181.70 × 10−60.864
    Br2.08 × 10−50.6171.61 × 10−60.863
    Kr1.93 × 10−50.6171.52 × 10−60.862
    Rb1.78 × 10−50.6161.44 × 10−60.862
    Sr1.65 × 10−50.6161.36 × 10−60.861
    Y1.53 × 10−50.6161.29 × 10−60.861
    Zr1.43 × 10−50.6161.22 × 10−60.861
    Nb1.33 × 10−50.6161.15 × 10−60.861
    Mo1.24 × 10−50.6161.09 × 10−60.861
    Table 3. Fitting coefficients according to Eqs. (3.20) and (3.21) for DR into He-like ions originating from the 1s2lnl′ and 1s3lnl′ autoionizing levels, with Z = Zn − 1, m = 2, and l0 = 0. The numerical data include corrections for multiple decay channels (two channels for 1s2lnl′ and four channels for 1s3lnl′).
    1s22lnl′: α0 = 1s22sα = 1s22p1s23lnl′: α0 = 1s22sα = 1s23p
    ElementBdχdBdχd
    Be8.09 × 10−50.057 11.97 × 10−60.197
    B6.86 × 10−50.040 02.85 × 10−60.173
    C5.18 × 10−50.030 66.61 × 10−60.161
    N3.95 × 10−50.024 81.06 × 10−50.153
    O3.09 × 10−50.020 71.47 × 10−50.149
    F2.47 × 10−50.017 91.85 × 10−50.145
    Ne2.02 × 10−50.015 62.17 × 10−50.142
    Na1.69 × 10−50.013 92.41 × 10−50.140
    Mg1.43 × 10−50.012 62.57 × 10−50.138
    Al1.23 × 10−50.011 52.67 × 10−50.136
    Si1.07 × 10−50.010 52.71 × 10−50.135
    P9.43 × 10−60.009 812.69 × 10−50.133
    S8.41 × 10−60.009 142.60 × 10−50.131
    Cl7.57 × 10−60.008 582.53 × 10−50.130
    Ar6.87 × 10−60.008 092.42 × 10−50.128
    K6.25 × 10−60.007 722.31 × 10−50.127
    C5.76 × 10−60.007 362.19 × 10−50.126
    Sc5.35 × 10−60.007 042.09 × 10−50.124
    Ti5.00 × 10−60.006 771.97 × 10−50.123
    V4.67 × 10−60.006 581.86 × 10−50.122
    Cr4.42 × 10−60.006 371.76 × 10−50.120
    Mn4.20 × 10−60.006 201.66 × 10−50.119
    Fe4.02 × 10−60.006 051.57 × 10−50.118
    Co3.86 × 10−60.005 921.48 × 10−50.117
    Ni3.72 × 10−60.005 811.40 × 10−50.116
    Cu3.61 × 10−60.005 711.32 × 10−50.115
    Zn3.51 × 10−60.005 641.25 × 10−50.114
    Ga3.42 × 10−60.005 581.18 × 10−50.113
    Ge3.35 × 10−60.005 531.11 × 10−50.112
    As3.25 × 10−60.005 561.05 × 10−50.111
    Se3.20 × 10−60.005 549.96 × 10−60.110
    Br3.20 × 10−60.005 469.43 × 10−60.109
    Kr3.17 × 10−60.005 468.92 × 10−60.108
    Rb3.15 × 10−60.005 478.45 × 10−60.107
    Sr3.13 × 10−60.005 488.01 × 10−60.106
    Y3.12 × 10−60.005 517.59 × 10−60.105
    Zr3.11 × 10−60.005 547.20 × 10−60.105
    Nb3.11 × 10−60.005 586.83 × 10−60.104
    Mo3.11 × 10−60.005 636.48 × 10−60.103
    Table 4. Fitting coefficients according to Eqs. (3.20) and (3.21) for DR into Li-like ions originating from the 1s22lnl′ and 1s23lnl′ autoionizing levels, with Z = Zn − 2, m = 1, and l0 = 0. The numerical data include corrections for multiple decay channels (one channel for 1s22lnl′ and four channels for 1s23lnl′).
    1s23lnl′: α0 = 1s22pα = 1s23d1s24lnl′: α0 = 1s22pα = 1s24d
    ElementBdχdBdχd
    Be1.78 × 10−40.1401.88 × 10−50.190
    B2.99 × 10−40.1372.01 × 10−50.189
    C3.74 × 10−40.1352.04 × 10−50.188
    N4.44 × 10−40.1332.18 × 10−50.187
    O5.15 × 10−40.1312.35 × 10−50.187
    F5.52 × 10−40.1302.53 × 10−50.186
    Ne5.65 × 10−40.1282.67 × 10−50.185
    Na5.76 × 10−40.1272.88 × 10−50.181
    Mg5.73 × 10−40.1253.28 × 10−50.174
    Al5.61 × 10−40.1243.32 × 10−50.172
    Si5.39 × 10−40.1223.33 × 10−50.171
    P5.19 × 10−40.1203.48 × 10−50.167
    S4.96 × 10−40.1193.46 × 10−50.165
    Cl4.71 × 10−40.1173.44 × 10−50.164
    Ar4.48 × 10−40.1153.41 × 10−50.163
    K4.25 × 10−40.1143.38 × 10−50.161
    C4.04 × 10−40.1123.34 × 10−50.160
    Sc3.83 × 10−40.1103.30 × 10−50.159
    Ti3.64 × 10−40.1093.25 × 10−50.158
    V3.45 × 10−40.1073.20 × 10−50.157
    Cr3.27 × 10−40.1053.14 × 10−50.156
    Mn3.11 × 10−40.1043.08 × 10−50.156
    Fe2.95 × 10−40.1023.02 × 10−50.155
    Co2.80 × 10−40.1012.95 × 10−50.154
    Ni2.66 × 10−40.09922.88 × 10−50.154
    Cu2.53 × 10−40.09782.80 × 10−50.153
    Zn2.40 × 10−40.09642.72 × 10−50.153
    Ga2.28 × 10−40.09512.64 × 10−50.153
    Ge2.17 × 10−40.09392.56 × 10−50.152
    As2.06 × 10−40.09272.47 × 10−50.152
    Se1.96 × 10−40.09162.39 × 10−50.152
    Br1.86 × 10−40.09052.30 × 10−50.152
    Kr1.77 × 10−40.08952.22 × 10−50.152
    Rb1.68 × 10−40.08852.14 × 10−50.152
    Sr1.60 × 10−40.08762.05 × 10−50.152
    Y1.52 × 10−40.08671.97 × 10−50.152
    Zr1.45 × 10−40.08591.89 × 10−50.152
    Nb1.38 × 10−40.08511.82 × 10−50.152
    Mo1.31 × 10−40.08441.74 × 10−50.152
    Table 5. Fitting coefficients according to Eqs. (3.20) and (3.21) for DR into excited states of Li-like ions originating from the 1s23lnl′ and 1s24lnl′ autoionizing levels, with Z = Zn − 2, m = 1, and l0 = 1. The numerical data include corrections for multiple decay channels (three channels for 1s23lnl′ and six channels for 1s24lnl′).
    StateZn = 3Zn = 6Zn = 13Zn = 18Zn = 26Zn = 42
    2p21S08.4 × 10105.1 × 10121.3 × 10131.9 × 10133.4 × 10137.0 × 1013
    2p21D21.5 × 10142.5 × 10143.1 × 10143.1 × 10142.3 × 10142.1 × 1014
    2p23P02.9 × 1072.3 × 1092.3 × 10111.2 × 10123.7 × 10122.8 × 1012
    2p23P1000000
    2p23P1 with Breit interaction2.6 × 1076.8 × 1081.9 × 10107.2 × 10103.2 × 10112.2 × 1012
    2p23P21.1 × 1093.1 × 10103.0 × 10122.1 × 10131.1 × 10141.5 × 1014
    Table 6. Field-free autoionization decay rates (s−1) including intermediate coupling, configuration, and magnetic interaction.
    F. B. Rosmej, V. A. Astapenko, V. S. Lisitsa, L. A. Vainshtein. Dielectronic recombination in non-LTE plasmas[J]. Matter and Radiation at Extremes, 2020, 5(6): 064201
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