Research Progress on Low-dimensional Halide Perovskite Direct X-ray Detectors

Siyin DONG; Shujie TIE; Ruihan YUAN; Xiaojia ZHENG

doi:10.15541/jim20230016

Journals >Journal of Inorganic Materials >Volume 38 >Issue 9 >Page 1017 > Article

Journal of Inorganic Materials
Vol. 38, Issue 9, 1017 (2023)

Research Progress on Low-dimensional Halide Perovskite Direct X-ray Detectors

Siyin DONG¹, Shujie TIE¹, Ruihan YUAN^1,2, and Xiaojia ZHENG^1,2,*

Author Affiliations

¹1. Institute of Chemical Materials, China Academy of Engineering Physics, Mianyang 621900, China

²2. Sichuan Research Center of New Materials, Chengdu 610200, China

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DOI: 10.15541/jim20230016 Cite this Article

Siyin DONG, Shujie TIE, Ruihan YUAN, Xiaojia ZHENG. Research Progress on Low-dimensional Halide Perovskite Direct X-ray Detectors[J]. Journal of Inorganic Materials, 2023, 38(9): 1017 Copy Citation Text

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1. Schematic diagram of (a) indirect and (b) direct X-ray detection^[33⇓-35]

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2. Schematic representation of the molecular structures of halide perovskites with different dimensions^[17]

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3. 0D bismuth-based perovskite single crystal detector

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4. 1D and 2D bismuth-based perovskite single crystal detectors

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5. 2D perovskite X-ray detectors

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6. Quasi-2D polycrystalline X-ray detector

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Compound	E_ph/keV,V_p/kV_p	Thickness/mm	Electric field/(V·mm^-1)	Sensitivity/(µC·Gy_air⁻¹·cm⁻²)	LoD/(nGy_air·s⁻¹)	Resistivity/(Ω·cm)	Bandgap/eV	µτ/(cm²·V⁻¹)	Ref.
Single crystal
Cs₄PbI₆	30 keV	-	-	451.49	90	-	3.46	9.7×10^-4	[55]
Cs₃Bi₂I₉	40 kV_p	1.2	50	1652.3	130	2.79×10¹⁰	1.96	7.97×10^-4	[28]
Cs₃Bi₂I₉	45 keV	1	120	964	44.6	1.12×10⁹	~1.89	1.87×10^-3	[53]
MA₃Bi₂i₉	100 kV_p	2.5	48	10620	0.62	5.27×10¹¹	1.98	2.8×10^-3	[25]
MA₃Bi₂i₉	40 kV_p	1	60	1947	83	3.74×10¹⁰	1.99	2.87×10^-3	[54]
FA₃Bi₂I₉	45 keV	0.9	~560	598.1	200	7.8×10¹⁰	2.08	2.4×10^-5	[52]
(DMEDA)BiI₅	50 kV_p	0.6	494	72.5	-	-	1.82	-	[58]
(H₂MDAP)BiI₅	70 keV	2	5	1.0	-	2.1×10¹⁰	1.83	-	[57]
CsPbI₃	50 kV_p	-	4.17	2370	3020	7.4×10⁹	2.67	3.63×10^-3	[59]
(NH₄)₃Bi₂I₉(∥001)	22 keV	-	2.2	8200	210	-	2.05	1.1×10^-2	[29]
(NH₄)₃Bi₂I₉ (⊥001)	22 keV	-	6.5	803	55	-	2.05	4.0×10^-3	[29]
Rb₃Bi₂I₉	30 keV	1	300	159.7	8.32	2.3×10⁹	1.89	2.51×10^-3	[61]
(F-PEA)₂PbI₄	120 keV	1.5	~130	3402	23	1.36×10¹²	2.30	5.1×10^-4	[66]
(PMA)₂PbI₄	40 kV_p	0.9	~56	283	2130	-	2.01	8.05×10^-3	[67]
BA₂PbI₄	30 kV_p	2	10	148	241	2.6×10¹¹	2.24	4.5×10^-4	[64]
BA₂CsPbBr₇	40 kV_p	3.91	2.53	13260	72.5	2.2×10⁹	2.74	-	[68]
BA₂EA₂Pb₃Br₁₀	70 keV	2	5	6.8×10³	5500	4.5×10¹⁰	2.55	1.0×10^-2	[69]
(CH₃OC₃H₉N)₂CsPb₂Br₇	80 kV_p	2	0	410	-	-	2.51	3.2×10^-3	[70]
BDAPbI₄	40 kV_p	-	310	242	430	-	2.37	4.43×10^-4	[72]
(BDA)CsPb₂Br₇	50 kV_p	0.7	~43	725.5	3810	4.35×10¹⁰	2.76	2.33×10^-5	[73]
(3AMPY)(FA)Pb₂I₇	50 kV_p	1	200	5.23×10⁴	151	-	1.54	2.0×10^-3	[75]
Polycrystalline
MA₃Bi₂i₉	35.5 keV	1	210	563	9.3	2.28×10¹¹	2.08	4.6×10^-5	[77]
MA₃Bi₂i₉	30.6 keV	~0.1	150	~35	140	~5×10¹¹	2.09	3.89×10^-5	[78]
MA₃Bi₂i₉	30.6 keV	~0.05	600	~100	98.4	3.38×10¹¹	2.03	1.6×10^-6	[79]
MA₃Bi₂i₉	40 kV_p	0.1	2000	2065	2.71	3.5×10⁸	1.86	-	[80]
Cs₄PbBr₆	-	0.3	666.7	7068	1.75	1.376×10¹¹	3.88	1.01×10^-3	[81]
Cs₂TeI₆	40 kV_p	0.025	25	19.2	-	4.2×10¹⁰	1.57	5.2×10^-5	[82]
BA₂MA₉Pb₁₀I₃₁	~60 keV	0.9	110	5362.3	8.1	~1×10¹⁰	~1.60	3.99×10^-5	[26]
BA₂MA₉Pb₁₀I₃₁	45 keV	1	210	7109	9.3	~1.1×10¹⁰	~1.61	~5×10^-5	[22]
(BA₂PbBr₄)_0.5FAPbI₃	-	0.006	~167	1.36×10⁴	4.2	-	-	-	[83]
PEA₂MA₈Pb₉I₂₈	50 kV_p	-	600	10 860	69	5.4×10¹⁰	1.504	2.6×10⁻⁵	[84]

Table 1. Comparison of low-dimensional perovskite X-ray detectors

Siyin DONG, Shujie TIE, Ruihan YUAN, Xiaojia ZHENG. Research Progress on Low-dimensional Halide Perovskite Direct X-ray Detectors[J]. Journal of Inorganic Materials, 2023, 38(9): 1017

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