• Chinese Physics B
  • Vol. 29, Issue 9, (2020)
Shuo Li, Lei Shi, and Zu-Wei Yan
Author Affiliations
  • College of Science, Inner Mongolia Agricultural University, Hohhot 010018, China
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    DOI: 10.1088/1674-1056/ab961a Cite this Article
    Shuo Li, Lei Shi, Zu-Wei Yan. Optical properties of core/shell spherical quantum dots[J]. Chinese Physics B, 2020, 29(9): Copy Citation Text show less

    Abstract

    In this study, the effects of quantum dot size on the binding energy, radiative lifetime, and optical absorption coefficient of exciton state in both GaN/AlxGa1-xN core/shell and AlxGa1-xN/GaN inverted core/shell quantum dot structures are studied. For the GaN/AlxGa1-xN core/shell structure, the variation trend of binding energy is the same as that of radiation lifetime, both of which increase first and then decrease with the increase of core size. For AlxGa1-xN/GaN inverted core/shell structure, the binding energy decreases first and then increases with core size increasing, and the trends of radiation lifetime varying with core size under different shell sizes are different. For both structures, when the photon energy is approximately equal to the binding energy, the peak value of the absorption coefficient appears, and there will be different peak shifts under different conditions.
    H^x=22meΔe+22mhΔh+Ue+Uhe24πε0ε|\boldsymbolre\boldsymbolrh|,(1)

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    H^x=22me(2re2+2rere+rerh+rehrereh×2rereh+2reh2+2rehreh)+22mh(2rh2+2rhrh+rhre+rehrhreh×2rhreh+2reh2+2rehreh)+Ue+Uhe24πε0εreh.(2)

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    Ue,h={0,re,hR1,Ve,h,R1re,hR2,,re,hR2,(3)

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    Ue,h={Ve,h,re,hR1,0,R1re,hR2,,re,hR2.(4)

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    Ve=0.6(Eg(AlxGa1xN)Eg(GaN)),(5)

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    Vh=0.4(Eg(AlxGa1xN)Eg(GaN)),(6)

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    Eg(AlxGa1xN)=(1x)Eg(GaN)+xEg(AlN).(7)

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    mi={mi1,ri<R1,mi2,R1riR2,(8)

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    me(AlxGa1xN)=(1x)me(GaN)+xme(AlN),(9)

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    mh(AlxGa1xN)=(1x)mh(GaN)+xmh(AlN),(10)

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    ε={ε1,reR1and  rhR1,ε2,  R1reR2  and  R1rhR2,ε1+ε22,  others.(11)

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    ϕi(r)={Ai1sin[ki1ri]ri,riR1,Ai2sinh[ki2(riR2)]ri,R1riR2,(12)

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    ϕi(r)={Ai1sinh[ki1ri]ri,riR1,Ai2sin[ki2(riR2)]ri,R1riR2,(13)

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    H^xΨ(re,rh,reh)=ExΨ(re,rh,reh).(14)

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    Ψx(re,rh,reh)=ϕe(re)ϕh(rh)eλreh,(15)

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    Ex=minλΨx|Hx|ΨxΨx|Ψx.(16)

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    Eb=Ee+EhEx.(17)

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    σ=πe2Ep6ncε0m0ωVIopδ(Ebω),(18)

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    Iop=|Ψx(re,rh,reh)δ(re,rh)dV|2.(19)

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    δ(Ebω)=Γπ[(Ebω)2+Γ2],(20)

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    f=Ep2EphIop.(21)

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    τ=6πε0m0c32e2nβsEph2f,(22)

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    Eph=Eg+Ex,(23)

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    βs=3εεNQD+2ε,(24)

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    Shuo Li, Lei Shi, Zu-Wei Yan. Optical properties of core/shell spherical quantum dots[J]. Chinese Physics B, 2020, 29(9):
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