• Journal of Radiation Research and Radiation Processing
  • Vol. 41, Issue 1, 010101 (2023)
Jianwei ZHANG1, Bo TIAN1, Jinfeng LI1, Zhigang LI1, Nan ZHANG1, Tuo LI1, Zhixin LIU1、2, Yuanjie SUN1, and Hongtao ZHAO1、*
Author Affiliations
  • 1Heilongjiang Institute of Atomic Energy, Harbin 150081, China
  • 2Yantai Research Institute of Harbin Engineering University, Yantai 264006, China
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    DOI: 10.11889/j.1000-3436.2022-0099 Cite this Article
    Jianwei ZHANG, Bo TIAN, Jinfeng LI, Zhigang LI, Nan ZHANG, Tuo LI, Zhixin LIU, Yuanjie SUN, Hongtao ZHAO. Research progress of amidoxime uranium adsorption materials[J]. Journal of Radiation Research and Radiation Processing, 2023, 41(1): 010101 Copy Citation Text show less
    Mechanism diagram of amidoxime preparation by cyano-hydroxylamine method
    Fig. 1. Mechanism diagram of amidoxime preparation by cyano-hydroxylamine method
    Amide (thioamide) -hydroxylamine method preparation-AO typical material[21]
    Fig. 2. Amide (thioamide) -hydroxylamine method preparation-AO typical material[21]
    Preparation of amidoxime functionalized ZIF-90-AO[31]
    Fig. 3. Preparation of amidoxime functionalized ZIF-90-AO[31]
    Reaction mechanism of PAO alkali treatment[45]
    Fig. 4. Reaction mechanism of PAO alkali treatment[45]
    Schematic illustration of the synthesis of In-Nx-C-R[70]
    Fig. 5. Schematic illustration of the synthesis of In-Nx-C-R[70]
    (a) Structure of amidoxime-functionalized layered porous polymer[56]; (b) diagram of U(VI) adsorption on PAN-NH2-AO[17]
    Fig. 6. (a) Structure of amidoxime-functionalized layered porous polymer[56]; (b) diagram of U(VI) adsorption on PAN-NH2-AO[17]
    Adsorption mechanism of MIL-101-SMA-AO[83]
    Fig. 7. Adsorption mechanism of MIL-101-SMA-AO[83]
    Three nucleophilic centers of amidoxime group[88]
    Fig. 8. Three nucleophilic centers of amidoxime group[88]
    Coordination modes of amidoxime ligands with metal ions[89]
    Fig. 9. Coordination modes of amidoxime ligands with metal ions[89]

    吸附剂

    Adsorption

    固液比 / (g·L-1)

    Solid-liquid

    ratio

    初始铀浓度 / (mg·L-1)

    Initial uranium

    concentration

    pH

    平衡时间 / min

    Equilibrium

    time

    最大吸附容量 / (mg·g-1)

    Maximum adsorption

    capacity

    文献

    Reference

    AGH0.5001006.0120398.40[58]
    semi-IPN-PAO0.010326.036 0001 279±14.50[59]
    KTG0.010355.0360512.60[60]
    PAO-CB0.0051286.01 9201 466.98[51]
    PAMSA3.0005003.030039.50[61]
    NC-PAO-DN0.010166.02 880465±27.00[62]
    CP-PAO0.005168.09 600465±26.36[63]
    GO-CMC-AO0.5001006.0120327.86[64]
    GO-CS-AO0.5001006.0120248.75[64]
    Zn2+-PAO0.005328.05 7601 188±18.90[57]
    GMPAO-105.060386.61[65]
    ZIF-90-AO0.1001005.090500.00[31]
    PAO@CHM0.015326.01 4401 091.53[66]
    Fe@PDA-PAO0.005767.02 7601 086.00[67]
    PAO-h-PEI0.050506.02 160985.70[68]
    Table 1. Adsorption performance of amidoxime functional gel adsorbents
    Jianwei ZHANG, Bo TIAN, Jinfeng LI, Zhigang LI, Nan ZHANG, Tuo LI, Zhixin LIU, Yuanjie SUN, Hongtao ZHAO. Research progress of amidoxime uranium adsorption materials[J]. Journal of Radiation Research and Radiation Processing, 2023, 41(1): 010101
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