• Chinese Journal of Lasers
  • Vol. 48, Issue 21, 2101006 (2021)
Tiancheng Zheng1、3, Xianglong Cai1、2, Zhonghui Li1, Chencheng Shen1、3, Dong Liu1, Jingbo Liu1、*, and Jingwei Guo1、**
Author Affiliations
  • 1Key Laboratory of Chemical Lasers, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian, Liaoning 116023, China
  • 2School of Science, Changchun University of Science and Technology, Changchun, Jilin 130022, China
  • 3University of Chinese Academy of Sciences, Beijing 100049, China
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    DOI: 10.3788/CJL202148.2101006 Cite this Article Set citation alerts
    Tiancheng Zheng, Xianglong Cai, Zhonghui Li, Chencheng Shen, Dong Liu, Jingbo Liu, Jingwei Guo. Visible Broadband Raman Lasers of H2∶CH4∶CO2 Gas Mixture Pumped by 532-nm Laser[J]. Chinese Journal of Lasers, 2021, 48(21): 2101006 Copy Citation Text show less
    Schematic diagram of stimulated Raman scattering experimental setup
    Fig. 1. Schematic diagram of stimulated Raman scattering experimental setup
    Steady-state Raman gain coefficients for H2, CO2, and CH4 varying with gas pressure.(a)Forward direction; (b)backward direction
    Fig. 2. Steady-state Raman gain coefficients for H2, CO2, and CH4 varying with gas pressure.(a)Forward direction; (b)backward direction
    Curves of energy conversion efficiency of each order Raman component of three gases varying with pressure. (a) H2; (b) CH4; (c) CO2
    Fig. 3. Curves of energy conversion efficiency of each order Raman component of three gases varying with pressure. (a) H2; (b) CH4; (c) CO2
    Energy conversion efficiency of each order Raman component of three gases varying with pump energy. (a) H2; (b) CH4; (c) CO2
    Fig. 4. Energy conversion efficiency of each order Raman component of three gases varying with pump energy. (a) H2; (b) CH4; (c) CO2
    Curves of conversion efficiency of main Raman light varying with pump energy and laser spectrum in gas mixture. (a) Variation curve; (b) laser spectrogram
    Fig. 5. Curves of conversion efficiency of main Raman light varying with pump energy and laser spectrum in gas mixture. (a) Variation curve; (b) laser spectrogram
    Energy level diagram and phase matching diagram for 853 nm laser generation by four-wave mixing. (a) Energy level diagram; (b) phase matching diagram
    Fig. 6. Energy level diagram and phase matching diagram for 853 nm laser generation by four-wave mixing. (a) Energy level diagram; (b) phase matching diagram
    GasΔυR /cm-1dσdΩ/10-31cm2·Sr-1gFR/cm·GW-1gBR/cm·GW-1
    H2Forward:0.0112/p+1.58p×10-3Backward:1.768/p+1.58p×10-37.92.1570.0161
    CH40.32+0.0118×pa270.2360.0645
    CO20.005773×pa2. 52b0.2170.0061
    Table 1. Parameters related to Raman gain of H2,CH4 and CO2 at 25 ℃ and 0.5 MPa
    Wavelength /nmIdentificationWavelength /nmIdentification
    435AS1(H2,532 nm)683S1 (H2, 532 nm)
    461AS1 (CH4, 532 nm)690S1 (CH4,574 nm); S1 (CO2, 630 nm)
    495AS1 (CO2, 532 nm)754S1 (H2,574 nm); S1 (CO2, 683 nm)
    532S0(pump)771S2 (CH4, 532 nm)
    574S1 (CO2, 532 nm)853S1 (H2,630 nm); S1 (CH4, 683 nm)
    624*S2 (CO2, 532 nm)954S2 (H2, 532 nm)
    630*S1 (CH4, 532 nm)
    Table 2. Output wavelengths of Raman laser in mixed gas
    Tiancheng Zheng, Xianglong Cai, Zhonghui Li, Chencheng Shen, Dong Liu, Jingbo Liu, Jingwei Guo. Visible Broadband Raman Lasers of H2∶CH4∶CO2 Gas Mixture Pumped by 532-nm Laser[J]. Chinese Journal of Lasers, 2021, 48(21): 2101006
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