• Acta Physica Sinica
  • Vol. 69, Issue 17, 173401-1 (2020)
Zhong-Huo Ling1、2, Shuai Wang2、5, Jin-Cang Zhang1, Yi-Zhu Zhang2、3、*, Tian-Min Yan2、*, and Yu-Hai Jiang2、4、5、*
Author Affiliations
  • 1Materials Genome Institute, Department of Physics, Shanghai University, Shanghai 200444, China
  • 2Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai 201210, China
  • 3Center for Terahertz Waves, College of Precision Instrument and Optoelectronics Engineering, Tianjin University, Tianjin 300072, China
  • 4University of Chinese Academy of Sciences, Beijing 100049, China
  • 5ShanghaiTech University, Shanghai 201210, China
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    DOI: 10.7498/aps.69.20200218 Cite this Article
    Zhong-Huo Ling, Shuai Wang, Jin-Cang Zhang, Yi-Zhu Zhang, Tian-Min Yan, Yu-Hai Jiang. The theoretical study of terahertz-streaking photoionization for ultrafast imaging of density matrix in rubidium atom[J]. Acta Physica Sinica, 2020, 69(17): 173401-1 Copy Citation Text show less
    Schematic diagram of terahertz-streaking photoioniza-tion experiments. (a) The probe pulses consist of a ultraviolet pulse and a terahertz pulse. The ultraviolet pulse is locked at the zero point of terahertz vector potential. The superposition state of rubidium atoms is excited by an infrared pulse. (b) Schematic diagram in energy representation. First, the electrons in the superposition state of rubidium atoms are ionized by a UV femtosecond pulse to form two characteristic spectral lines in the photoelectron energy spectrum. Second, the continuous electron with different final momenta is driven by the terahertz pulse. The spectral lines are broadened and the interference occurs.
    Fig. 1. Schematic diagram of terahertz-streaking photoioniza-tion experiments. (a) The probe pulses consist of a ultraviolet pulse and a terahertz pulse. The ultraviolet pulse is locked at the zero point of terahertz vector potential. The superposition state of rubidium atoms is excited by an infrared pulse. (b) Schematic diagram in energy representation. First, the electrons in the superposition state of rubidium atoms are ionized by a UV femtosecond pulse to form two characteristic spectral lines in the photoelectron energy spectrum. Second, the continuous electron with different final momenta is driven by the terahertz pulse. The spectral lines are broadened and the interference occurs.
    The evolution of photoelectron momentum spectra as a function of time delay: (a) Photoelectron momentum spectra without a terahertz field; (b) photoelectron momentum spectra with a terahertz field.
    Fig. 2. The evolution of photoelectron momentum spectra as a function of time delay: (a) Photoelectron momentum spectra without a terahertz field; (b) photoelectron momentum spectra with a terahertz field.
    Time-domain resolution of quantum coherence and the reconstruction of density matrix: (a) Coherent dynamics of the quantum system. The solid line is the theoretical prediction of the coherence term. The dotted line is the cross section along the blue line in Fig. 2 (b) to extract the phase information. (b) Yellow line is the photoelectron momentum distribution driven by THz electric field at . The red line represents the population contribution; and the green line represents the coherence contribution.
    Fig. 3. Time-domain resolution of quantum coherence and the reconstruction of density matrix: (a) Coherent dynamics of the quantum system. The solid line is the theoretical prediction of the coherence term . The dotted line is the cross section along the blue line in Fig. 2 (b) to extract the phase information. (b) Yellow line is the photoelectron momentum distribution driven by THz electric field at . The red line represents the population contribution; and the green line represents the coherence contribution.
    Zhong-Huo Ling, Shuai Wang, Jin-Cang Zhang, Yi-Zhu Zhang, Tian-Min Yan, Yu-Hai Jiang. The theoretical study of terahertz-streaking photoionization for ultrafast imaging of density matrix in rubidium atom[J]. Acta Physica Sinica, 2020, 69(17): 173401-1
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