• Chinese Journal of Lasers
  • Vol. 50, Issue 1, 0113015 (2023)
Haoran Long1、2, Yuan Gao3, Hao Liu1、2, Kaiyao Xin1、2, Yali Yu1、2, Juehan Yan1、2、*, and Zhongming Wei1、2、**
Author Affiliations
  • 1State Key Laboratory of Superlattices and Microstructures, Institute of Semiconductors, Chinese Academy of Sciences, Beijing 100083, China
  • 2Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China
  • 3Center of Military Commission Equipment Development Department, Beijing 100032, China
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    DOI: 10.3788/CJL221103 Cite this Article Set citation alerts
    Haoran Long, Yuan Gao, Hao Liu, Kaiyao Xin, Yali Yu, Juehan Yan, Zhongming Wei. Ultraviolet Photodetector Based on Wide Bandgap Two-Dimensional Semiconductor TlGaS2[J]. Chinese Journal of Lasers, 2023, 50(1): 0113015 Copy Citation Text show less
    Crystal structure and material characterization results. (a) TlGaS2 crystal structure; (b) optical microscope photos of nanosheets; (c) AFM test; (d) Raman test result; XPS test results of elements (e) Tl and (f) Ga
    Fig. 1. Crystal structure and material characterization results. (a) TlGaS2 crystal structure; (b) optical microscope photos of nanosheets; (c) AFM test; (d) Raman test result; XPS test results of elements (e) Tl and (f) Ga
    Theoretical calculation and absorption spectrum test results. (a) Energy band structure of TlGaS2 bulk material; (b) density of states at band edge; (c) measured absorption spectrum of TlGaS2 nanosheet
    Fig. 2. Theoretical calculation and absorption spectrum test results. (a) Energy band structure of TlGaS2 bulk material; (b) density of states at band edge; (c) measured absorption spectrum of TlGaS2 nanosheet
    Test results of photoelectric performances of TlGaS2 photodetector. (a) Structural diagram of TlGaS2 detector; (b) output curves under dark state and different wavelength light irradiation conditions with optical microscope photo of device shown in insert; (c) spectral response range of detector; (d) responsivity and specific detection rate versus wavelength; (e) transient response test results under different optical power densities at 360 nm; (f) photocurrent versus optical power density
    Fig. 3. Test results of photoelectric performances of TlGaS2 photodetector. (a) Structural diagram of TlGaS2 detector; (b) output curves under dark state and different wavelength light irradiation conditions with optical microscope photo of device shown in insert; (c) spectral response range of detector; (d) responsivity and specific detection rate versus wavelength; (e) transient response test results under different optical power densities at 360 nm; (f) photocurrent versus optical power density
    Working performances and principle of TlGaS2 photodetector. (a) Response speed; (b) noise performance under weak field; (c) air stability; (d) photocurrent two-dimensional plane scanning test; (e)(f) working principle of detector
    Fig. 4. Working performances and principle of TlGaS2 photodetector. (a) Response speed; (b) noise performance under weak field; (c) air stability; (d) photocurrent two-dimensional plane scanning test; (e)(f) working principle of detector
    MaterialWavelength /nmResponsivity /(mA·W-1Response time(rise/delay)Reference

    CuGaS2

    PbI2

    FePS3

    GaPS4

    BiOBr

    Bi2O3

    GeSe2

    h-BN

    GaN

    Ga2O3

    ZnO

    TlGaS2

    254

    375

    254

    254

    315

    300

    355

    212

    360

    254

    370

    360

    5.1×103

    510

    170

    791

    1.2×107

    2.21×103

    127

    0.1

    251

    39.3

    10.5

    57

    1.8 s/10.1 s

    14.1 ms/31.0 ms

    105 ms/120 ms

    ~50 ms

    110 μs/160 μs

    290 μs/870 μs

    <30 ms

    320 ms/630 ms

    1.12 ms/2.80 ms

    84.83 s/219.19 s

    1.4 s/6.8 s

    51.8 μs/45.1 μs

    37

    38

    39

    4

    5

    19

    40

    20

    41

    42

    43

    This work

    Table 1. Performance comparison of ultraviolet photodetectors based on wide bandgap materials
    Haoran Long, Yuan Gao, Hao Liu, Kaiyao Xin, Yali Yu, Juehan Yan, Zhongming Wei. Ultraviolet Photodetector Based on Wide Bandgap Two-Dimensional Semiconductor TlGaS2[J]. Chinese Journal of Lasers, 2023, 50(1): 0113015
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