• Optical Instruments
  • Vol. 43, Issue 1, 49 (2021)
Tengfei ZHANG, Debao ZHANG, Yuhong ZHANG, and Guanjun YOU*
Author Affiliations
  • School of Optical-Electrical and Computer Engineering, University of Shanghai for Science and Technology, Shanghai 200093, China
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    DOI: 10.3969/j.issn.1005-5630.2021.01.008 Cite this Article
    Tengfei ZHANG, Debao ZHANG, Yuhong ZHANG, Guanjun YOU. Study on the three-photon nonlinear optical absorption of all-inorganic perovskite CsPbBr3 nanoplatelets[J]. Optical Instruments, 2021, 43(1): 49 Copy Citation Text show less

    Abstract

    CsPbBr3 nanoplatelets (NPLs) with different thickness (3-5 monolayers) were synthesized by ligand-assisted reprecipitation at room temperature to study the nonlinear optical absorption properties in the near-infrared-II window. The nonlinear three-photon absorption properties of CsPbBr3 NPLs were investigated by Z-scan technique using a laser with central wavelength of 1030 nm, pulse width of 6 ps and repetition of 25 kHz. The experimental results show that the nonlinear three-photon absorption cross section of CsPbBr3 NPLs is significantly increased due to the enhancement of quantum confinement effect with decreasing the thickness of NPLs. The three-photon absorption cross section of the 3 monolayers NPLs is 4.1 × 10-71 cm6s2photon-2. This study shows that CsPbBr3 NPLs have excellent nonlinear multiphoton absorption properties in the near-infrared-II window, and can be applied in the field of multiphoton fluorescence imaging.
    $ \frac{{\rm{d}}I\left(z\right)}{{\rm{d}}z}=-{\alpha }_{3}{I}^{3}\left(z\right) $(1)

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    $ I\left(z,\lambda \right)=\frac{{I}_{0}\left(\lambda \right)}{\sqrt{1+2{\alpha }_{3}\left(\lambda \right){I}_{0}^{2}\left(\lambda \right)z}} $(2)

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    $ {T}_{\rm{OA}}=\dfrac{1}{{\left[1+2{\alpha }_{3}{L}_{\rm{eff}}{\left(\dfrac{{I}_{0}}{1+{\left(\dfrac{z}{{z}_{0}}\right)}^{2}}\right)}^{2}\right]}^{\frac{1}{2}}} $(3)

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    $ {\sigma }_{3}\left(\lambda \right)={\sigma }_{3}'\left(\lambda \right)\times {\left(\left(h\upsilon \right)\right)}^{2} $(4)

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    $ {\sigma }_{3}'\left(\lambda \right)={\alpha }_{3}\left(\lambda \right)/\left({N}_{\rm{A}}{d}_{0}\right) $(5)

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    Tengfei ZHANG, Debao ZHANG, Yuhong ZHANG, Guanjun YOU. Study on the three-photon nonlinear optical absorption of all-inorganic perovskite CsPbBr3 nanoplatelets[J]. Optical Instruments, 2021, 43(1): 49
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