• Chinese Optics Letters
  • Vol. 21, Issue 12, 120021 (2023)
Wanchen Tao1, Siqi Sun1, Lixin He1,*, Yanqing He1..., Jianchang Hu1, Yu Deng1, Chengqing Xu1, Pengfei Lan1,** and Peixiang Lu1,2|Show fewer author(s)
Author Affiliations
  • 1Wuhan National Laboratory for Optoelectronics and School of Physics, Huazhong University of Science and Technology, Wuhan 430074, China
  • 2Hubei Key Laboratory of Optical Information and Pattern Recognition, Wuhan Institute of Technology, Wuhan 430205, China
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    DOI: 10.3788/COL202321.120021 Cite this Article Set citation alerts
    Wanchen Tao, Siqi Sun, Lixin He, Yanqing He, Jianchang Hu, Yu Deng, Chengqing Xu, Pengfei Lan, Peixiang Lu, "Measurement of molecular alignment with deep learning-based M-XFROG technique [Invited]," Chin. Opt. Lett. 21, 120021 (2023) Copy Citation Text show less
    References

    [1] L. Cai, J. Marango, B. Friedrich. Time-dependent alignment and orientation of molecules in combined electrostatic and pulsed nonresonant laser fields. Phys. Rev. Lett., 86, 775(2001).

    [2] H. Stapelfeldt, T. Seideman. Colloquium: aligning molecules with strong laser pulses. Rev. Mod. Phys., 75, 543(2003).

    [3] O. Ghafur, A. Rouzée, A. Gijsbertsen, W. K. Siu, S. Stolte, M. J. J. Vrakking. Impulsive orientation and alignment of quantum-state-selected NO molecules. Nat. Phys., 5, 289(2009).

    [4] Y. Ohshima, H. Hasegawa. Coherent rotational excitation by intense nonresonant laser fields. Int. Rev. Phys. Chem., 29, 619(2010).

    [5] K. Lin, I. Tutunnikov, J. Qiang, J. Ma, Q. Song, Q. Ji, W. Zhang, H. Li, F. Sun, X. Gong, H. Li, P. Lu, H. Zeng, Y. Prior, I. Sh. Averbukh, J. Wu. All-optical field-free three-dimensional orientation of asymmetric-top molecules. Nat. Commun., 9, 5134(2018).

    [6] E. T. Karamatskos, S. Raabe, T. Mullins, A. Trabattoni, P. Stammer, G. Goldsztejn, R. R. Johansen, K. Długołecki, H. Stapelfeldt, M. J. J. Vrakking, S. Trippel, A. Rouzée, J. Küpper. Molecular movie of ultrafast coherent rotational dynamics of OCS. Nat. Commun., 10, 3364(2019).

    [7] I. V. Litvinyuk, K. F. Lee, P. W. Dooley, D. M. Rayner, D. M. Villeneuve, P. B. Corkum. Alignment-dependent strong field ionization of molecules. Phys. Rev. Lett., 90, 233003(2003).

    [8] T. K. Kjeldsen, C. Z. Bisgaard, L. B. Madsen, H. Stapelfeldt. Role of symmetry in strong-field ionization of molecules. Phys. Rev. A, 68, 063407(2003).

    [9] J. Wu, H. Cai, H. Zeng, A. Couairon. Femtosecond filamentation and pulse compression in the wake of molecular alignment. Opt. Lett., 33, 2593(2008).

    [10] R. A. Bartels, T. C. Weinacht, N. Wagner, M. Baertschy, C. H. Greene, M. M. Murnane, H. C. Kapteyn. Phase modulation of ultrashort light pulses using molecular rotational wave packets. Phys. Rev. Lett., 88, 013903(2001).

    [11] J. Itatani, J. Levesque, D. Zeidler, H. Niikura, H. Pépin, J. C. Kieffer, P. B. Corkum, D. M. Villeneuve. Tomographic imaging of molecular orbitals. Nature, 432, 867(2004).

    [12] C. Vozzi, M. Negro, F. Calegari, G. Sansone, M. Nisoli, S. De Silvestri, S. Stagira. Generalized molecular orbital tomography. Nat. Phys., 7, 822(2011).

    [13] C. Zhai, X. Zhang, X. Zhu, L. He, Y. Zhang, B. Wang, Q. Zhang, P. Lan, P. Lu. Single-shot molecular orbital tomography with orthogonal two-color fields. Opt. Express, 26, 2775(2018).

    [14] L. He, X. Zhu, W. Cao, P. Lan, P. Lu. Attosecond spectroscopy for filming the ultrafast movies of atoms, molecules and solids. Chin. Phys. B, 31, 123301(2022).

    [15] R. Velotta, N. Hay, M. B. Mason, M. Castillejo, J. P. Marangos. High-order harmonic generation in aligned molecules. Phys. Rev. Lett., 87, 183901(2001).

    [16] J. Itatani, D. Zeidler, J. Levesque, M. Spanner, D. M. Villeneuve, P. B. Corkum. Controlling high harmonic generation with molecular wave packets. Phys. Rev. Lett., 94, 123902(2005).

    [17] T. Kanai, S. Minemoto, H. Sakai. Ellipticity dependence of high-order harmonic generation from aligned molecules. Phys. Rev. Lett., 98, 053002(2007).

    [18] O. Smirnova, Y. Mairesse, S. Patchkovskii, N. Dudovich, D. Villeneuve, P. Corkum, M. Y. Ivanov. High harmonic interferometry of multi-electron dynamics in molecules. Nature, 460, 972(2009).

    [19] L. He, P. Lan, A. T. Le, B. Wang, B. Wang, X. Zhu, P. Lu, C. D. Lin. Real-time observation of molecular spinning with angular high-harmonic spectroscopy. Phys. Rev. Lett., 121, 163201(2018).

    [20] P. M. Kraus, B. Mignolet, D. Baykusheva, A. Rupenyan, L. Horný, E. F. Penka, G. Grassi, O. I. Tolstikhin, J. Schneider, F. Jensen, L. B. Madsen, A. D. Bandrauk, F. Remacle, H. J. Wörner. Measurement and laser control of attosecond charge migration in ionized iodoacetylene. Science, 350, 790(2015).

    [21] L. He, S. Sun, P. Lan, Y. He, B. Wang, P. Wang, X. Zhu, L. Li, W. Cao, P. Lu, C. D. Lin. Filming movies of attosecond charge migration in single molecules with high harmonic spectroscopy. Nat. Commun., 13, 4595(2022).

    [22] A. Rupenyan, J. B. Bertrand, D. M. Villeneuve, H. J. Wörner. All-optical measurement of high-harmonic amplitudes and phases in aligned molecules. Phys. Rev. Lett., 108, 033903(2012).

    [23] Y. He, L. He, P. Lan, B. Wang, L. Li, X. Zhu, W. Cao, P. Lu. Direct imaging of molecular rotation with high-order-harmonic generation. Phys. Rev. A, 99, 053419(2019).

    [24] B. Wang, L. He, Y. He, Y. Zhang, R. Shao, P. Lan, P. Lu. All-optical measurement of high-order fractional molecular echoes by high-order harmonic generation. Opt. Express, 27, 30172(2019).

    [25] Y. Huang, J. Zhao, Z. Shu, Y. Zhu, J. Liu, W. Dong, X. Wang, Z. Lü, D. Zhang, J. Yuan, J. Chen, Z. Zhao. Ultrafast hole deformation revealed by molecular attosecond interferometry. Ultrafast Sci., 2021, 9837107(2021).

    [26] Y. Chen, X. Zhu, P. Lan, P. Lu. Background-free detection of molecular chirality using a single-color beam [Invited]. Chin. Opt. Lett, 20, 100004(2022).

    [27] E. Péronne, M. D. Poulsen, C. Z. Bisgaard, H. Stapelfeldt, T. Seideman. Nonadiabatic alignment of asymmetric top molecules: field-free alignment of iodobenzene. Phys. Rev. Lett., 91, 043003(2003).

    [28] P. Huber-Wälchli, D. M. Guthals, J. W. Nibler. Cars spectra of supersonic molecular beams. Chem. Phys. Lett., 67, 233(1979).

    [29] M. D. Duncan, P. Österlin, R. L. Byer. Pulsed supersonic molecular-beam coherent anti-Stokes Raman spectroscopy of C2H2. Opt. Lett., 6, 90(1981).

    [30] T. Lang, M. Motzkus, H. M. Frey, P. Beaud. High resolution femtosecond coherent anti-Stokes Raman scattering: determination of rotational constants, molecular anharmonicity, collisional line shifts, and temperature. J. Chem. Phys., 115, 5418(2001).

    [31] T. Hornung, H. Skenderović, K.-L. Kompa, M. Motzkus. Prospect of temperature determination using degenerate four-wave mixing with sub-20 fs pulses. J. Raman Spectrosc., 35, 934(2004).

    [32] K. Yoshii, G. Miyaji, K. Miyazaki. Measurement of molecular rotational temperature in a supersonic gas jet with high-order harmonic generation. Opt. Lett., 34, 1651(2009).

    [33] Y. He, L. He, P. Wang, B. Wang, S. Sun, R. Liu, B. Wang, P. Lan, P. Lu. Measuring the rotational temperature and pump intensity in molecular alignment experiments via high harmonic generation. Opt. Express, 28, 21182(2020).

    [34] X. Guo, C. Jin, Z. He, J. Yao, X.-X. Zhou, Y. Cheng. Retrieval of molecular alignment and identification of multiple-orbital contribution by using polarized high harmonics from aligned N2 molecules. Opt. Express, 29, 1613(2021).

    [35] C. Jiang, H. Jiang, Y. Chen, B. Li, C. D. Lin, C. Jin. Genetic-algorithm retrieval of the molecular alignment distribution with high-order harmonics generated from transiently aligned CO2 molecules. Phys. Rev. A, 105, 023111(2022).

    [36] P. Wang, L. He, Y. He, J. Hu, S. Sun, P. Lan, P. Lu. Rotational echo spectroscopy for accurate measurement of molecular alignment. Opt. Lett., 47, 1033(2022).

    [37] P. Lu, J. Liu, H. Li, H. Pan, J. Wu, H. Zeng. Cross-correlation frequency-resolved optical gating by molecular alignment for ultraviolet femtosecond pulse measurement. Appl. Phys. Lett., 97, 061101(2010).

    [38] J. Liu, Y. Feng, H. Li, P. Lu, H. Pan, J. Wu, H. Zeng. Supercontinuum pulse measurement by molecular alignment based cross-correlation frequency resolved optical gating. Opt. Express, 19, 40(2011).

    [39] R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbügel, B. A. Richman, D. J. Kane. Measuring ultrashort laser pulses in the time-frequency domain using frequency-resolved optical gating. Rev. Sci. Instrum., 68, 3277(1997).

    [40] D. J. Kane, R. Trebino. Single-shot measurement of the intensity and phase of an arbitrary ultrashort pulse by using frequency-resolved optical gating. Opt. Lett., 18, 823(1993).

    [41] D. J. Kane. Real-time measurement of ultrashort laser pulses using principal component generalized projections. IEEE J. Sel. Top. Quantum Electron., 4, 278(1998).

    [42] C. Szegedy, W. Liu, Y. Jia, P. Sermanet, S. Reed, D. Anguelov, D. Erhan, V. Vanhoucke, A. Rabinovich. Going deeper with convolutions. IEEE Conference on Computer Vision and Pattern Recognition (CVPR)(2015).

    [43] J. White, Z. Chang. Attosecond streaking phase retrieval with neural network. Opt. Express, 27, 4799(2019).

    [44] T. Szidarovszky, M. Jono, K. Yamanouchi. LIMAO: cross-platform software for simulating laser-induced alignment and orientation dynamics of linear-, symmetric- and asymmetric tops. Comput. Phys. Commun., 228, 219(2018).

    [45] T. Seideman. Rotational excitation and molecular alignment in intense laser fields. J. Chem. Phys., 103, 7887(1995).

    [46] T. Seideman. On the dynamics of rotationally broad, spatially aligned wave packets. J. Chem. Phys., 115, 5965(2001).

    [47] Md. Z. Hoque, M. Lapert, E. Hertz, F. Billard, D. Sugny, B. Lavorel, O. Faucher. Observation of laser-induced field-free permanent planar alignment of molecules. Phys. Rev. A, 84, 013409(2011).

    [48] H. Li, W. Li, Y. Feng, H. Pan, H. Zeng. Field-free molecular orientation by femtosecond dual-color and single-cycle THz fields. Phys. Rev. A, 88, 013424(2013).

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    Wanchen Tao, Siqi Sun, Lixin He, Yanqing He, Jianchang Hu, Yu Deng, Chengqing Xu, Pengfei Lan, Peixiang Lu, "Measurement of molecular alignment with deep learning-based M-XFROG technique [Invited]," Chin. Opt. Lett. 21, 120021 (2023)
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