Ce-La@Fe3O4 composite adsorbents were fabricated by hydrothermal method and it was used to remove fluoride from aqueous solution. SEM images show that Ce-La@Fe3O4 adsorbents are square particle with diameter of (1.22±0.35) μm, and a certain extent adhesion are observed after the adsorption fluoride. The pseudo-second-order has been found suitable for describing the kinetics process of the fluoride absorption on Ce-La@Fe3O4 adsorbents while the net rate can thus be sequentially controlled in a multi-stage condition. The fitness of adsorption data by Langmuir model is superior to Freundlich model．The fluoride adsorption capacity would increase obviously when the reactive temperature rises. Ce-La@Fe3O4 adsorbents are magnetic, and are easy to be recovered and reused by ordinary magnets after adsorption fluoride.