Abstract
1 Introduction
Green lasers are of great interest in biomedicine, laser display, spectroscopy, underwater optical communications, and scientific research.1 In contrast to the well-developed red or blue laser diodes (LDs), LDs emitting directly in the green region are still under development and hence the “green gap” exists.2 Currently, the leading technology for producing high-power continuous-wave (CW) green lasers is still the nonlinear frequency conversion (e.g., frequency doubling) of near-infrared solid-state or fiber laser systems,3,4 and the compactness, stabilization, and expenditure are still challenges. As a result, researchers are always looking for an alternate green-light laser solution that has the benefits of great brightness, compactness, and cost-effectiveness. Due to intrinsic advantages, such as good beam quality, small footprint, user-friendliness, and low- to no-maintenance, green fiber lasers doped with trivalent rare-earthions (e.g., ,5,67) can satisfy these demands and bridge the “green gap,” so there is a huge drive to develop compact high-power rare-earth-doped fiber lasers in the green spectral region.
Given recent advances in both rare-earth-doped fluoride fibers and blue GaN LD, frequency down conversion fiber lasers using trivalent rare-earth-doped fluoride fibers have emerged as a promising approach to directly generate visible-light emission, and much related work has been carried out and reported.8
Herein, we designed and experimentally demonstrated a compact high-power all-fiber CW -doped green laser for the first time to our knowledge. To begin, an efficient butt-coupled all-fiber structure capable of high-power operation was constructed using a DC -doped fluoride fiber treated by the cutting process and fiber dichroic mirrors (FDMs) with a high damage intensity. Following that, to achieve high-efficiency emission and high-power output, we explored the effects of gain fiber length and output mirror reflectivity on green laser power scaling via experiments and numerical simulations. Finally, according to the optimization results, we designed and further presented an experimental study on the compact high-power green all-fiber laser, which comprises a 2.1-m DC -doped fluoride fiber, two FDMs at visible wavelengths, and a 443-nm fiber-pigtailed pump source. The laser can directly generate a 3616-mW green laser output with a central wavelength of and a slope efficiency of 18.8%.
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2 Experimental Principle and Setup
2.1 Spectroscopy of DC
First, we briefly discuss the spectroscopic properties of DC -doped fluoride fiber. The fiber is manufactured by Le Verre Fluoré and has the following features: a doping concentration of 8000 ppm, a core diameter, a 0.08-numerical aperture (NA) of fiber core, inner cladding (double D-shaped), and outer cladding diameter, respectively. The core cutoff wavelength of this gain fiber is 780 nm, and its V-parameter (normalized frequency) at 521 nm is about 3.6. We first measured the fiber attenuation spectrum (including doping absorption in the core and propagation loss in the inner cladding) at room temperature by a tungsten halogen lamp and a 350- to 1750-nm optical spectrum analyzer (OSA, AQ6315B, Ando), as shown in the inset of Fig. 1(a). The propagation loss spectrum is then estimated by fitting the data at different wavelengths (i.e., 1.10 dB/m at 543 nm, 0.88 dB/m at 650 nm, and 0.74 dB/m at 793 nm) [see the blue curve in the inset of Fig. 1(a)]. Finally, the ground state absorption of DC -doped fiber is obtained by deducting the propagation loss spectrum from the attenuation spectrum, as shown in Fig. 1(a). The peak absorption coefficient is 2.4 dB/m at 441 nm, while the absorption coefficient at our pump wavelength (i.e., 443 nm) is 2.1 dB/m. The absorption cross sections can be calculated based on Beer–Lambert’s law, and the related calculation equations are simply derived as follows:18,19
Figure 1.Spectroscopy of 8000 ppm DC
The simplified energy level scheme of for visible fluorescence emission is shown in Fig. 1(c). The frequency down conversion fluorescence emission in the green spectral region is known to emanate from the levels. The excitation process is as follows: (1) level is excited by ground state absorption of the level with the pump, (2) nonradiative relaxation from to , and (3) radiative transition from to , which can generate fluorescence emission at and .20Figure 1(d) shows the fluorescence emission spectrum of the 0.6-m DC -doped fluoride fiber excited by a 443-nm laser. The stimulated emission spectrum displays the emission lines in the deep red (), red (), orange (), green (), and blue () spectral regions, implying the potential of these different visible-wavelength fiber lasers. In addition, the emission cross sections are computed using the Füchtbauer–Ladenburg (F-L) theory, which is expressed as21,22
2.2 Experimental Setup
To construct an effective butt-coupled all-fiber structure capable of high-power operation in our experiment, we must first prepare the high-performance FC/PC fiber connectors at both ends of DC -doped fluoride fiber. At present, due to fragile mechanical properties of fluoride fiber, it is inevitable that the fiber end-facet will be damaged to some extent by the traditional polishing processing [see Fig. 2(a)], which leads to the lower damage intensity of the fiber end-facet and blocks high-power operation. Therefore, to enable visible high-power laser operation, a new reliable processing technology for fluoride fiber end-facet nondestructive processing must be developed. Continuous experiments have revealed that fluoride fiber cutting technology based on a commercial fiber cleaver (CT104+, Fujikura) combined with the fabrication technology of a standard FC/PC fiber connector can effectively solve the aforementioned issues. First, the fiber cleaver is used to cleave the fluoride fiber to obtain the fiber end-facet with high smoothness. The fiber is then inserted into the ceramic core with an inner diameter of until it is parallel to the end-facet of the ceramic core. Finally, a small amount of UV-curing adhesive is added to the end of the ceramic core for curing, and the DC -doped fluoride fiber connector with high smoothness is successfully prepared, as shown in Fig. 2(b). The above process skillfully applies the fiber cutting technology to fabricate the high-quality fluoride fiber connector and ensures the construction of an effective all-fiber structure capable of high-power operation. Furthermore, to obtain high-performance FDMs at visible wavelengths, heat-resistant epoxy resin combined with grinding and polishing technology is first utilized to produce fiber end-facets with high stability and smoothness. The main processes are as follows: (1) producing the silica fiber connector by using the ceramic core and heat-resistant epoxy resin; (2) solidifying the fiber connector at high temperature; and (3) grinding and polishing the end-facet of the solidified fiber connector by a commercial polishing machine. The FDMs at visible wavelengths with high laser damage intensity () are then successfully prepared using an ion beam-assisted deposition system and a specific electric field manipulation of film layers, which is also one of the key factors for achieving high-power green all-fiber lasers.
Figure 2.Microscopic images of DC
After finishing the processing of the fluoride fiber connector and the preparation of FDMs with high damage intensity, we designed the all-fiber -doped green laser. The schematic of green laser is shown in Fig. 3(a), and Fig. 3(b) shows the corresponding photograph. This laser consists of a DC -doped fluoride fiber, two FDMs, and a 443-nm pump source. The pump can deliver 20-W pump power at 443 nm through a standard multimode (0.22 NA) silica fiber pigtail. Two ceramic sleeves with a 2.5-mm inner diameter are used to realize the low-loss all-fiber coupling between the DC -doped fluoride fiber and the visible FDMs. The compact fiber linear cavity for green-light oscillation is constructed by two homemade FDMs (, ). The FDM was fabricated by directly coating the dielectric films onto the end-facet of standard multimode silica fiber. The reflectivity of is as high as 99.7% at 521 nm, and it has a high transmittance of 95.4% at 443 nm [see Fig. 3(c)]. The reflectivity of and is 74.9% and 87.2% at 521 nm, respectively, and both have a high reflectivity of at 443 nm [see Fig. 3(c)], which ensures the sufficient utilization of the residual pump laser. All FDMs are designed to have a high transmittance at 635 nm to suppress red laser emission. The propagation loss of the pump laser through the DC -doped fluoride fiber is measured to be 1.45 dB/m [see the inset of Fig. 1(a)], whereas the loss of the core is estimated to be at 521 nm.10 In addition, the green laser was measured by the OSA (AQ-6315E, Ando), and the output power was recorded by a 350- to 1100-nm optical power meter (S425C-L, Thorlabs, Inc.).
Figure 3.(a) Schematic and (b) photograph of the compact all-fiber
3 Results and Discussion
3.1 High-Power All-Fiber Green Laser
According to the optimization results, a DC -doped fluoride fiber and were employed for the high-power all-fiber green laser experiment. Figure 4 exemplifies the output characteristics of the green laser. The threshold of the CW green laser is about 1030 mW. Figure 4(a) shows the green output power at different pump powers. With the increase of pump power, the output power increases linearly without saturation, and the slope efficiency is 18.8%. Accordingly, a maximum output power of 3616 mW was attained pumped at 20.01 W. The wide range of the output spectrum at 5.71 W pump power is shown in Fig. 4(b). Note that the central wavelength of the spectrum is 521.2 nm, and the intensity of the green laser is higher than that of the residual pump laser, indicating that of the output laser is green laser. The spectra of the green laser under different pump powers are given in Fig. 4(c). With the increase of pump power, the center wavelength of the green laser shows a slight redshift, and the 3-dB spectral bandwidth also expands. Under strong pumping, the green laser oscillates at multiple wavelengths and has a wide spectral bandwidth due to the design of a high cavity in a wide reflective waveband [see Fig. 4(c)]. As shown in Fig. 4(d), to evaluate the operation stability of the all-fiber green laser, we monitored the power curve of the green laser operating at 3.0 W for over 60 min. The intensity fluctuation is , showing the excellent long-term stability of the laser operation. In addition, the laser intensity distribution and factors of the generated green fiber laser beam were measured by a beam quality analyzer (WinCamD-UCD12, DataRay), and the measurement results are shown in the inset of Fig. 4(d). The measured parameters are 4.99 and 4.25, respectively, indicating that the green fiber laser is multitransverse mode operation.
Figure 4.Characteristics of the high-power all-fiber green laser. (a) Output green power versus the pump power. (b) Typical spectrum collected from 400 to 800 nm under 5.71 W pump power. (c) Output spectra under different pump powers. (d) Power stability curve of the green laser operating at 3.0 W. Insets: the beam quality parameters and intensity distribution of the green laser.
3.2 Output Characteristics of All-Fiber Green Lasers with Different Designs
The output characteristics of the all-fiber green lasers with different designs were investigated experimentally, as shown in Fig. 5. Figure 5(a) shows the green laser power versus the pump power with the different gain fiber lengths () and the laser reflectivity () of . For the reflectivity of 74.9%, varying the gain fiber from 4 to 1.9 m, both the green output power and slope efficiency increase from 536 to 830 mW pumped at 5.07 W and from 13.0% to 20.9%, respectively. When , with decreasing from 87.2% to 74.9%, both the green output power and slope efficiency increase from 801 to 1344 mW pumped at 7.63 W and from 11.9% to 20.9%, respectively. Figure 5(b) shows the corresponding green spectra pumped at 3.76 W. The results show that all the all-fiber green lasers with different designs oscillate at multiple wavelengths under strong pumping. Along with higher green power, the linewidth of the green laser becomes broadening and new wavelengths are emitted at the edge of the fluorescence spectrum. According to the comparison experiment with different designs, the output performance of the all-fiber green laser with DC -doped fiber and output coupling is superior.
Figure 5.Characteristics of the all-fiber green laser with different designs. (a) Output green power versus the pump power and (b) the corresponding spectra pumped at 3.76 W.
3.3 Numerical Analysis
To better understand and further optimize the performance of the all-fiber -doped green laser, numerical simulations of this laser were carried out. The laser transition process of in is a typical four-level system, which can be simulated using the numerical model of the strongly pumped quasi-four-level laser system, as shown in Fig. 6. This model focuses on the correlation transitions among the four energy levels of [i.e., (), (), (), and ()]. In this case, the steady-state rate equations and power transmission equations can be expressed as follows:23
Figure 6.Numerical model. (a) Typical four-level system and (b) schematic of end-pumped fiber laser.
Parameter | Value | Parameter | Value |
443 nm | |||
521 nm | |||
0 | 0.92 | ||
0 | Variable | ||
4% | |||
99% | |||
95% | |||
Variable |
Table 1. The parameters used in numerical simulation.
Figure 7.Simulation performance of the all-fiber green laser. (a) Output power as a function of the
Figure 8.(a) Green output power as a function of the pump power for different
As visualized in Fig. 7(a), for a fixed input pump power, the laser output power first increases and then falls as the gain fiber length increases. The figure also reveals that with the decrease of , the of gain fiber realizing the maximum output power becomes longer. Figure 7(b) shows the laser threshold and slope efficiency of the green fiber laser versus the under , . A maximum slope efficiency is 23.3% at , yielding a laser threshold of 0.84 W. For the designed laser (, ), although there exists an optimum fiber length (), sufficient pump absorption should be considered to ensure that the remaining reverse pump laser does not affect the pump source, and the gain fiber is thus selected in high-power laser experiment. Figures 7(c) and 7(d) show the laser output power, slope efficiency, and threshold versus the under , . It can be seen the output power first increases and then decreases with the reducing of under a fixed pump power. As the pump increases, the laser reflectivity for maximum power output decreases [see the dotted arrow in Fig. 7(c)]. As shown in Fig. 7(d), with the increase of , the laser threshold and slope efficiency decrease. It is worth mentioning, however, that in DC -doped fluoride fiber, the emission cross section of red light is substantially bigger than that of green light (i.e., the red gain is much stronger than that of green light). Even with only feedback at both ends of the resonant cavity, red laser oscillation is easily formed under vigorous pumping. In practice, with the decrease of (i.e., the threshold of green laser increases), red laser oscillation may be established first in the -doped fiber laser, resulting in the failure of green laser emission. Therefore, in designing the output mirror reflectivity of an all-fiber -doped green laser, various factors (e.g., gain fiber length, output mirror transmittance in the red region) should be considered comprehensively to ensure the successful establishment of green laser oscillation. For example, in experiment, a DC -doped fluoride fiber was used, and the threshold of the red laser is about 1.6 W without the FDMs. According to the green laser threshold in Fig. 7(d), it can be inferred that should be designed to be at this time to obtain higher efficiency and output power on the premise of the smooth establishment of the green laser.
We also carried out relevant simulations of the high-power all-fiber green laser with different optimization designs, and the results are shown in Fig. 8(a). For the , varying the gain fiber from 2.1 to 1.5 m, both the green output power and slope efficiency increase from 3.63 to 4.23 W pumped at 20 W and from 19.0% to 22.1%, respectively. When the , with the decreasing from 75% to 50%, both the green output power and slope efficiency increase from 3.63 to 5.41 W pumped at 20 W and from 20.5% to 30.0%, respectively. Therefore, the output power and efficiency can be further improved by reasonably reducing the length of the gain fiber and increasing the green laser output coupling. Furthermore, as shown in Fig. 8(b), neglecting the loss caused by a higher doping level, it can be found that the green laser output power increases with the increase of the doping concentration, indicating that the output green laser power can also be further increased by increasing the doping concentration. In short, the numerical model well explains the experimental results of the all-fiber green laser [see the black sphere in Figs. 7(b), 7(d), and 8(a)], and predicts the potential of the visible DC -doped all-fiber laser pumped by a standard multimode fiber-pigtailed blue LD.
4 Conclusions
A compact high-efficiency Watt-level CW all-fiber -doped green laser pumped by a 443-nm fiber-pigtailed pump source was demonstrated. To achieve high-efficiency and high-power operation, the DC -doped fluoride fiber connector was processed based on the cutting technology, and then the all-fiber green laser design was optimized using experiments and numerical simulations. According to the optimization results, we designed and demonstrated a compact high-power green all-fiber laser, which consists of a 2.1-m DC -doped fiber, two homemade FDMs at visible wavelengths with a high damage intensity, and a 443-nm fiber-pigtailed pump source. The maximum output green laser power is up to 3.62 W at 521 nm, and the maximum slope efficiency is as high as 20.9%. To the best of our knowledge, this is the largest output power from the visible fiber lasers so far. Simulation performance of all-fiber green laser also shows that it is necessary to consider the optimum gain fiber length, output mirror reflectivity, and doping level. We believe the laser power scaling and slope efficiency could be further improved via (1) reducing the reflectivity of the output mirror at the laser wavelength, (2) uprating the power of 443 nm fiber-pigtailed pump laser, and (3) reducing the propagation loss and enhancing the doping level of DC -doped fiber.
Jinhai Zou received his BS degree in optoelectronic information science and engineering from China Jiliang University in 2017 and his PhD in electronic science and technology from Xiamen University in 2022. His research focuses on fiber lasers in the visible waveband.
Zhengqian Luo received his BS degree in applied physics from Harbin Institute of Technology in 2004 and his PhD in electrical engineering from Xiamen University in 2009. From 2007 to 2009, he studied at Nanyang Technological University as a joint PhD student. He joined Xiamen University as a faculty member in 2010. From 2016 to 2017, he was a visiting professor at Massachusetts Institute of Technology. Since 2017, he has been a full professor at Xiamen University and currently serves as the head of the Electronic Engineering Department of Xiamen University. His research focuses on ultrafast fiber lasers and on-chip photonic devices. He has published more than 150 journal or conference papers with total citations of >5500 times. He is a recipient of the National Science Fund for Excellent Young Scholars and the Fujian Youth Science and Technology Award. He is a senior member of IEEE and serves as a young editorial board member of Chinese Laser Press and associate director of the Optical Society of Fujian Province of China.
Biographies of the other authors are not available.
References
[14] J. Zou et al. Towards visible-wavelength passively mode-locked lasers in all-fibre format. Light Sci. Appl., 9, 61(2020).
[17] J. Nakanishi et al. Watt-order direct green laser oscillation at 522 nm in Pr3+-doped waterproof fluoro-aluminate-glass fiber, JTu4A.02(2013).
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