• NUCLEAR TECHNIQUES
  • Vol. 45, Issue 11, 110201 (2022)
Tao ZHANG1、2, Ke HAN1、2, Jianglai LIU1、2, Yue MENG1、2、*, Yukun YAO1, Siguang WANG3, Bobo LI4, Yinqi LIU4, and Teng PEI4
Author Affiliations
  • 1Sichuan Research Institute, Shanghai Jiao Tong University, Chengdu 610213, China
  • 2School of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240, China
  • 3School of Physics, State Key Laboratory of Nuclear Physics and Technology and Center for High Energy Physics, Peking University, Beijing 100871, China
  • 4Luoyang Shuangrui Titanium Precision Casting Co. , Ltd. , Luoyang 471000, China
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    DOI: 10.11889/j.0253-3219.2022.hjs.45.110201 Cite this Article
    Tao ZHANG, Ke HAN, Jianglai LIU, Yue MENG, Yukun YAO, Siguang WANG, Bobo LI, Yinqi LIU, Teng PEI. Investigation of vacuum melting technique for low background titanium[J]. NUCLEAR TECHNIQUES, 2022, 45(11): 110201 Copy Citation Text show less

    Abstract

    Background The expected signal rate of rare decay experiments, such as instance dark matter and neutrino less double beta decay experiments, is extremely low, which requires that the detector building materials have extremely low radioactivity. Low radioactive background control is one of the essential works in the rare decay experiments. 226Ra and 228Ra produced in the early decay chain of 238U and 232Th have low boiling point and high vapor pressure, removing the element Ra can break the 238U decay chain and keep a low radioactivity of 232Th-late for a long time. Purpose This study aims to investigate vacuum melting technique for low background titanium to reduce the impurity of isotopes that have negative impact on rare decay experiments and creating a low background environment for the detector running. Methods Firstly, the low background material samples were acquired by manual separation of radionuclides using physical and chemical methods. Then, radioactive impurity elements, such as K, Cs, Ra, Pb, Po and Rn with low boiling point and high vapor pressure, were volatilized in environment with high temperature and high vacuum level. Finally, radioactivity of these testing samples were measured by two sets of high-purity germanium γ spectrometer with measurement time extended to 7 days. Results Measurement results show signs of removal of radioactive isotopes by smelting-vacuum method, and the impurity in pure titanium smelted in vacuum electron beam furnace can reach the levels of (0.13±0.69) mBq∙kg-1 for 232Th-228Ac, and (0.07±0.29) mBq∙kg-1 for 238U-222Rn, respectively. Conclusions The smelting-vacuum method could provide reliable low background material for the container of the next generation PandaX detector.
    Tao ZHANG, Ke HAN, Jianglai LIU, Yue MENG, Yukun YAO, Siguang WANG, Bobo LI, Yinqi LIU, Teng PEI. Investigation of vacuum melting technique for low background titanium[J]. NUCLEAR TECHNIQUES, 2022, 45(11): 110201
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