Abstract
1. INTRODUCTION
Optical modulators play a crucial role in photonic integrated circuits (PICs) for optical interconnection and computation under the circumstance of ever-growing data traffic [1–3]. In recent years, a variety of electro-optic modulators have been reported, which are implemented on several platforms such as an InGaAsP/Si hybrid metal-oxide–semiconductor [4,5] and classical nonlinear crystals that include lithium niobate [6,7]. However, most of these modulators have issues of large footprint (tens or hundreds of micrometer level) or limited modulation-speed at the GHz level. Over the past few years, all-optical modulators have emerged with higher operating speeds than their electronic counterparts [8,9]. Yet, the weak photon–photon interaction remains an impediment for all-optical device design. Thus, for higher compactness and efficiency, optimized photonic structures with strong optical nonlinear interaction are necessary. Currently, epsilon-near-zero (ENZ) materials that exhibit a vanishing real part of the permittivity in a certain wavelength range have emerged with ultrahigh nonlinear response [10]. As a key member of ENZ materials, ITO has been extensively applied in optical modulators with its active electro-variable refractive index [11–13]. However, the large optical third-order nonlinearity from ITO at the ENZ region, which may bring large modulation depth and high modulation speed, has hardly been utilized in modulators hitherto. Moreover, in addition to the nonlinear coefficient of the material itself, efficient nonlinearity is also affected by the photonic structural design. Under this circumstance, recent exploration of the enhanced sensitivity from an exceptional point (EP) in parity-time (PT) symmetry theory may offer a novel approach.
The concept of PT symmetry effectively describes the existence of completely real spectra for non-Hermitian Hamiltonians with complex conjugation potential as [14]. PT-symmetric Hamiltonians can undergo a phase transition to a symmetry-broken regime, where complex eigenvalues appear formally through a parametric variation [15]. This kind of transition point could be manifested by the properties of EP, which are initiated in the studying of non-Hermitian operators. At the EP, both the eigenvalues and eigenstates coalesce [16]. It has been proved that an elaborate parametric design would lead systems to operate around EP and exhibit enhanced sensitivity [17–20]. For the past decade, non-Hermitian physics and PT symmetry have prompted novel micro-nano devices with high performance, for instance, nonreciprocal resonators [21,22], PT-symmetric lasers [23,24], and non-Hermitian electromagnetic metasurfaces [25]. Tunable effects of PT symmetry have exhibited signs of applications, including 1D and 2D photonic lattice geometries through tuning the complex refractive index [26–28], single-mode laser through manipulating the gain/loss of a microring resonator [29], and light-light switching through interferometrical manipulation [30]. However, most of these cases contain the gain media that are difficult to be applied in high-speed all-optical control [31–33]. Further, PT symmetry theory has yet to be practically introduced into the design of nonlinear all-optical modulators. It is known that, during the optimization of a modulator, plenty of attempts and simulations are always repeated with different geometric parameters in order to attain the optimum performance. By contrast, the EP may reasonably explicate the optimizing process and make it straightforward to improve the modulation depth and reduce the device footprint.
Here, we propose a non-Hermitian all-optical modulator based on PT symmetry utilizing the large optical nonlinearity from ITO in its ENZ region to tune the coupling coefficient between two waveguides. This optical modulator is designed to operate around EP and achieve THz-level switching through an external femtosecond pump laser, leading to the advantages of nanoscale integration, large modulation-depth, and high-speed all-optical control. To the best of our knowledge, it is the first time that the practical application based on PT symmetry is demonstrated for nonlinear all-optical modulators. The presented structure is composed of conventional materials such as silicon and cobalt, which have good compatibility toward CMOS fabrication technologies. Also, our work identifies a method of optimization for nanostructures using PT symmetry theory, which could be directly extended to the PIC platform and provides a new impetus for the development of all-optical applications.
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2. THEORY DEMONSTRATION AND THE PROPOSED MODULATOR
Figure 1.Coupled-waveguides system with its representation of the complex eigenvalues as Riemannian surfaces. (a) Two coupled waveguides, as lossless and lossy ones, respectively, form an integrated system that possesses a Hamiltonian
The proposed modulator integrated on substrate is presented in Fig. 2(a), which comprises an ITO layer sandwiched by a lossless propagating waveguide and a hybrid lossy waveguide. The propagating waveguide is totally composed of silicon (), while the hybrid lossy waveguide consists of silicon () and cobalt. Here, cobalt is exploited to break through the limitation of Kramers–Kronig relations owing to its similar real part of refractive index to silicon and a large extinction coefficient, which reduces the detuning between two waveguides while leading to heavy loss [38,39]. In order to utilize the large Kerr coefficient from ITO and distinguish the signal and pump, the signal wavelength is set as 1240 nm (ENZ wavelength), while the pump is chosen at 1250 nm according to one of the previous reports on ITO’s Kerr nonlinearity, where the change of the refractive index is from to with 30° incident pump [40]. Note that the operating wavelength at 1240 nm is deduced from current data, and this wavelength could be moved to 1550 nm telecom wavelength through changing ITO’s annealing temperature and doping concentration [41]. In our work, ITO is expected to realize the alteration of a coupling coefficient through its different refractive index with and without the pump laser. With regard to the modulation mechanism, on the one hand, ITO would involve in the light–matter interaction when a pump laser is applied, leading to an increased real part of refractive index and a decreased imaginary part. With the reduced difference between the refractive indexes of ITO and silicon, propagating light will be coupled into the hybrid lossy waveguide and decay consequently, which results in an off-state. On the other hand, the system is working on-state without a pump. These two states are plotted as power-flow at and planes, as shown in Figs. 2(b) and 2(c). Apparently, a portion of power-flow is distributed in ITO and the hybrid lossy waveguide at the off-state, indicating the light-field coupling and sharp attenuation. Here, the on-state transmitted power efficiency (the ratio of output and input power) is about 50.69%, while the off-state one is 10.68%, which gives the extinction ratio of 6.46 dB.
Figure 2.Schematics of the proposed modulator, internal electric-field, and power-flow distribution. (a) Structure of modulator integrated on
It has been proved that, for an ITO–air interface case, the electric-field components (normal to the interface) in ITO are inversely proportional to the permittivity of ITO because of the continuous displacement field; thus, the electric field would be enhanced at the ENZ region with an obliquely incident light [40]. The calculation result of electric-field enhancement in ITO at the plane is shown in Fig. 2(d). The maximum electric-field enhancement inside ITO reaches up to 31 times, and the average enhancement is about 14 times. This enhancement boosts the third-order optical nonlinear interactions in ITO, contributing to enlarging the variation of the linear refractive index at lower pumping power [42]. Note that the nonlinear optical coefficients of silicon [43] and cobalt [44] are several orders of magnitude smaller than that of ITO at the ENZ wavelength; thus, the nonlinear responses of silicon and cobalt are not under consideration.
3. RESULTS AND SYSTEM ANALYSIS
For the whole system of the non-Hermitian modulator, here the conventional coupled-mode-theory is used (see Appendix C for its reasonability in this system), and the optical-field dynamics can be represented by coupled mode equations as
To search for the EP, the simulation of -dependent transmitted power efficiency of the propagating waveguide with and without a pump has been carried out and plotted, as shown in Fig. 3(a). In order to keep the approximation () valid, the sum of and the width of are set to be invariant, which means the condition of is always the same. Clearly, the dashed and solid blue curves decrease sharply when reaches up to 160 nm. Further, the ascending transmission efficiency above 224 nm induced by the increasing loss corresponds to the “loss-induced transparency” [36]. It can be inferred that EP should be around 224 nm where the extinction ratio reaches the maximum. Note that the abnormal increasing trend of the transmitted power efficiency before 160 nm is mainly caused by the influence of the gap mode as produced in (see in Appendix B). To study the coupling mechanism around EP, the quantitative calculation for coupling coefficient with and without pump is plotted in Fig. 3(b). For a better comparison, the coupling-coefficient ratio (division of coefficients with pump and without pump) is calculated and shown as the red curves. The coupling-coefficient ratio around EP presents a sharp peak, corresponding to an increase of extinction ratio.
Figure 3.Analysis of PT-symmetric and PT-broken regions and eigenvalue spectra of the whole modulator system. (a) Transmitted power efficiency varies with
To further verify the accurate location of EP, calculation for propagation loss is absolutely necessary. Considering the existence of attenuation at on-state (mainly caused by loss of ITO), an approximative approach is adopted to divide ITO in half and distribute them into two waveguides (see in Appendix C for the calculation method). Then, the propagation loss of a hybrid lossy waveguide is presented as , and the is for the propagation loss of the propagating waveguide caused by the half of ITO. The PT-symmetric and PT-broken regions attained from the comparison of and are plotted in Fig. 3(c) (without pump) and Fig. 3(d) (with pump). Deduced from the intersection point of the red and black curves, the location of EP has a change from 184 nm (without pump) to 201 nm (with pump). The system has been actually PT-broken, even when extinction ratio has not risen to the maximum. In fact, the sensitivity is significantly enhanced near the transition point from the PT-symmetric to PT-broken regime, not actually the EP [17]; further, the near-EP region has been commonly utilized in device design [46–48]. Thus, performing the mode switching or modulation operation does not require crossing the EP, and it would be reasonable to set modulator’s operating point at the PT-broken state (near EP) in consideration of high extinction ratio. Given all this, the real and imaginary spectra of systems’ eigenvalues with and without a pump have been calculated according to Eq. (6) in Figs. 3(e) and 3(f). For a better demonstration, here is utilized as the unit of horizontal coordinate-axis. The calculated results commendably match the analysis of Riemannian surfaces in Fig. 1.
The influence of on the modulator’s extinction ratio and on-state transmitted efficiency is studied as shown in Figs. 4(a) and 4(b). The trends of these two performance parameters are nearly opposite under the variation of (the larger extinction ratio, the lower on-state transmitted efficiency), which suggests that it should be necessary to balance these two parameters. Two ultimate situations when is 30 and 70 nm are plotted in Figs. 4(c) and 4(d). For the case of , the extinction ratio reaches 10.16 dB, and the on-state transmitted efficiency is 42.5% [Fig. 4(c)], while the extinction ratio is 3.19 dB with on-state transmitted efficiency up to 63.9% under 70 nm [Fig. 4(d)]. Another decisive factor of the overall performance of modulators is modulation speed. For our structure, the modulation speed mainly depends on the group velocity in the modulation region and lifetime of the nonlinear response. As the calculation process shows in Appendix D, the propagating time is about 21.2 fs, while the recovery time of the nonlinear response in ITO is 360 fs. Thus, the recovery time is the predominant factor, which allows an all-optical modulation speed up to 2.78 THz, promising for advancement of the terahertz modulators [49,50].
Figure 4.Analysis of the balance between extinction ratio and on-state transmitted efficiency. (a), (b) The
4. DISCUSSION AND CONCLUSION
As described, the offset between EP and the locations of maximum extinction ratio is an inevitable challenge due to the loss of tunable material. To overcome this problem, a new method may be possibly employed to replace ITO by multiple metallic-quantum-wells (MQWs) [51,52], which could largely enhance the optical nonlinearity at the lower-loss wavelength region. On the other hand, for our tentative structure that demonstrates the application of PT symmetry on nonlinear all-optical modulator, there is still room for improvement. For example, the hybrid lossy waveguide could be placed at both sides of the propagating waveguide to achieve shorter modulation length and a more compact device, while it will introduce the difficulty to analyze the coupling coefficient at the same time. In addition, it is also reasonable to consider the resonant ring structure [53] to further improve the performance. Furthermore, the plasmonic structures with extreme field-confinement may prospectively contribute to the advancement of extinction ratio [54,55]. In regard to fabrication of this non-Hermitian modulator, the silicon waveguide can be fabricated by the electron-beam lithography and etching process. The cobalt waveguide and ITO slot can be processed by the film deposition after the electron-beam lithography. These several rounds of processes are compatible with the standard CMOS technology, thus enabling the prospect of integration with other PIC platforms [56–58]. At last, due to the 14-times electric-field enhancement provided by the sandwich structure (waveguide, ITO, waveguide) at the ENZ wavelength, and comparing with four-times enhancement in Ref. [40], the actual requirement of incident intensity would be reduced to about . As an example of a femtosecond laser with 100 fs pulse width, 80 MHz repetition rate, and the focused spot radius of , the averaged power of 16.56 mW is supposed to be applied. Moreover, the transmitted efficiency versus pump intensity in Appendix A shows that the required power could be reduced further with slight sacrifice of extinction ratio.
In summary, we propose an all-optical modulator based on non-Hermitian PT symmetry utilizing the nonlinearity from ITO at the ENZ region. Further, it has been demonstrated that applying the supreme sensitivity around EP to the all-optical modulator would lead to performance improvement and superiority. For the presented structure, the modulation depth comes up to , while the on-state transmitted efficiency is 50.69%. Additionally, the modulator has a compact device footprint of and an ultrahigh modulation speed that is up to the THz level. Moreover, the proposed device commendably proves the practical application of EPs in on-chip integrated modulators, which would be referred and extended to the design methodology of various nanostructures and further prompt the development of all-optical communication and high-speed signal processing.
Acknowledgment
Acknowledgment. H. Q. and H. M. conceived the idea. H. M. conducted the numerical simulations. H. M., D. L., and H. Q. contributed extensively to the writing of the manuscript. H. M., D. L., N. W., Y. Z., H. C., and H. Q. analyzed data and interpreted the details of the results. H. C. and H. Q. supervised the research.
APPENDIX A: SIMULATION FOR THE WHOLE STRUCTURE
Numerical simulations using the finite element method, including the power flow in the waveguides, calculation of coupling coefficient, and loss coefficient, are performed with COMSOL Multiphysics. The 2D mode analysis presented as electric-field distribution for the input port of propagating waveguide is plotted in Fig.
Figure 5.Electric-field distribution of the input port for propagating waveguide.
Figure 6.Transmitted efficiency versus pump intensity.
APPENDIX B: GAP MODE ANALYSIS
Figure
Figure 7.Normalized electric-field distributions in the hybrid lossy waveguide. (a) Schematic of the whole system at the
APPENDIX C: CALCULATION METHOD FOR COUPLING COEFFICIENT AND PROPAGATION LOSS
The modulator’s Hamiltonian is deduced from the coupled mode theory (CMT). Actually, using the conventional CMT for the coupled-waveguides here may cause 1% to 2% error according to Ref. [
For the non-Hermitian PT-symmetry system, loss and the real part of refractive index are equally important; further, the coupling coefficient should be calculated at the existence of cobalt. Here, the coupling coefficient is normally characterized by the coupling length, which is defined as the distance where the maximum guided power is transferred from one waveguide to the other. Accordingly, the coupling coefficient can be represented as
Figure 8.Normalized transmitted power in hybrid lossy waveguide that is used for calculation of coupling coefficients. (a) Schematic of the simulation structure. The red cross section in hybrid lossy waveguide is used to calculate the surface integral of power flow at each location. (b), (c) Situations without and with pump, respectively. The
Figure 9.Simulation structures for the calculation of propagation loss and their normalized transmitted power (as the example when ITO is under pump). (a) The propagating waveguide with a half of ITO. (b) The hybrid lossy waveguide with a half of ITO. The imaginary part of the refractive index in the left part (marked as lossless part by gray dashed rectangle) is deliberately set to be zero for the more realistic simulation of the propagating and coupling mechanism, which leads to a sharp decay when light propagates to hybrid lossy waveguide. (c), (d) The decay curves of the transmitted power in (a) and (b). The initial positions (
APPENDIX D: MODULATION SPEED
For the presented modulator, the modulation speed generally depends on the propagation time in the modulation region and the lifetime of nonlinear response. The speed of propagation could use the concept group velocity for the description. Group velocity can be interpreted as the speed of information in a wave, which is defined as [
Figure 10.Calculation for propagation speed, which is the ratio of the apparent change in
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