• Chinese Optics Letters
  • Vol. 20, Issue 9, 093701 (2022)
Tingyuan Jia1、2、3, Shaoming Xie1、2, Zeyu Zhang1、2、3、4、*, Qinxue Yin1、3, Chunwei Wang1、2、3、5, Chenjing Quan1、2, Xiao Xing1, Juan Du1、2、3、4、**, and Yuxin Leng1、2、3、5、***
Author Affiliations
  • 1State Key Laboratory of High Field Laser Physics and CAS Center for Excellence in Ultra-intense Laser Science, Shanghai Institute of Optics and Fine Mechanics (SIOM), Chinese Academy of Sciences (CAS), Shanghai 201800, China
  • 2Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China
  • 3Hangzhou Institute for Advanced Study, University of Chinese Academy of Sciences, Hangzhou 310024, China
  • 4School of Physics and Electronics, Shandong Normal University, Jinan 250014, China
  • 5School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China
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    DOI: 10.3788/COL202220.093701 Cite this Article Set citation alerts
    Tingyuan Jia, Shaoming Xie, Zeyu Zhang, Qinxue Yin, Chunwei Wang, Chenjing Quan, Xiao Xing, Juan Du, Yuxin Leng. Role of the interlayer interactions in ultrafast terahertz thermal dynamics of bilayer graphene[J]. Chinese Optics Letters, 2022, 20(9): 093701 Copy Citation Text show less
    (a) Schematic diagram of MLG on SiO2 substrate; (b) schematic diagram of BLG film on SiO2 substrate; (c) Raman spectra of MLG and BLG.
    Fig. 1. (a) Schematic diagram of MLG on SiO2 substrate; (b) schematic diagram of BLG film on SiO2 substrate; (c) Raman spectra of MLG and BLG.
    (a) Photoinduced THz conductivity of MLG and BLG as a function of the rising time at 1.91 eV, 160 µJ/cm2; (b) photoinduced THz conductivity of MLG and BLG as a function of the delay time at 1.91 eV, 160 µJ/cm2.
    Fig. 2. (a) Photoinduced THz conductivity of MLG and BLG as a function of the rising time at 1.91 eV, 160 µJ/cm2; (b) photoinduced THz conductivity of MLG and BLG as a function of the delay time at 1.91 eV, 160 µJ/cm2.
    (a)–(c) Relaxation process of MLG (black) and BLG (red) as a function of pump fluence at different photon energies; (d) relaxation process of MLG (black) and BLG (red) as a function of photon energy at the same pump fluence.
    Fig. 3. (a)–(c) Relaxation process of MLG (black) and BLG (red) as a function of pump fluence at different photon energies; (d) relaxation process of MLG (black) and BLG (red) as a function of photon energy at the same pump fluence.
    (a)–(c) Optical-induced THz conductivity peak value |Δσ| of MLG (black) and BLG (red) under different photon energies as a function of pump fluence; (d) ultrafast hot carrier cooling process of MLG and ultrafast heating and hot carrier cooling process of BLG. Diagrams of ultrafast processes and relaxation dynamics involving optical pumping (straight arrows), electron scattering (curled arrows), and optical phonon scattering (vertical blue wiggled arrows). Filled (open) circles signify electrons (holes). (e) Schematic diagram of the ultrafast dynamics in graphene after photoexcitation.
    Fig. 4. (a)–(c) Optical-induced THz conductivity peak value |Δσ| of MLG (black) and BLG (red) under different photon energies as a function of pump fluence; (d) ultrafast hot carrier cooling process of MLG and ultrafast heating and hot carrier cooling process of BLG. Diagrams of ultrafast processes and relaxation dynamics involving optical pumping (straight arrows), electron scattering (curled arrows), and optical phonon scattering (vertical blue wiggled arrows). Filled (open) circles signify electrons (holes). (e) Schematic diagram of the ultrafast dynamics in graphene after photoexcitation.
    (a), (b) Extracted frequency dependence of the THz conductivity at delay times of 0 ps and 2 ps for MLG, solid lines show the fit of the complex conductivity to a Drude model; (c), (d) extracted frequency dependence of the THz conductivity at delay times of 0 ps and 2 ps for BLG, solid lines show the fit of the complex conductivity to a Drude model.
    Fig. 5. (a), (b) Extracted frequency dependence of the THz conductivity at delay times of 0 ps and 2 ps for MLG, solid lines show the fit of the complex conductivity to a Drude model; (c), (d) extracted frequency dependence of the THz conductivity at delay times of 0 ps and 2 ps for BLG, solid lines show the fit of the complex conductivity to a Drude model.
     η at 0.78 eVη at 1.13 eVη at 1.91 eV
    MLG0.161±0.0430.198±0.0980.199±0.051
    BLG0.256±0.0680.320±0.0950.379±0.053
    Table 1. The Heating Parameter η
    Tingyuan Jia, Shaoming Xie, Zeyu Zhang, Qinxue Yin, Chunwei Wang, Chenjing Quan, Xiao Xing, Juan Du, Yuxin Leng. Role of the interlayer interactions in ultrafast terahertz thermal dynamics of bilayer graphene[J]. Chinese Optics Letters, 2022, 20(9): 093701
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